#------------------------------------------------------------------------------ #$Date: 2024-05-22 04:53:43 +0300 (Wed, 22 May 2024) $ #$Revision: 291979 $ #$URL: file:///home/coder/svn-repositories/cod/cif/2/02/31/2023136.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2023136 loop_ _publ_author_name 'Chi, Nguyen Thi Thanh' 'Van Thong, Pham' 'Thang, Nguyen Manh' 'Thao, Pham Ngoc' 'Van Meervelt, Luc' _publ_section_title ; Synthesis and crystal structures of three organoplatinum(II) complexes bearing natural arylolefin and quinoline derivatives ; _journal_coeditor_code PK2707 _journal_issue 6 _journal_name_full 'Acta Crystallographica Section E Crystallographic Communications' _journal_paper_doi 10.1107/S2056989024004572 _journal_volume 80 _journal_year 2024 _chemical_formula_iupac '[Pt (C15 H19 O4) Cl (C9 H7 N)]' _chemical_formula_moiety 'C24 H26 Cl N O4 Pt' _chemical_formula_sum 'C24 H26 Cl N O4 Pt' _chemical_formula_weight 623.00 _chemical_name_systematic ; Chlorido[4-methoxy-5-(2-oxo-2-propoxyethoxy)-2-(prop-2-en-1-yl)phenyl]\ (quinoline)platinum(II) ; _space_group_crystal_system monoclinic _space_group_IT_number 14 _space_group_name_Hall '-P 2ybc' _space_group_name_H-M_alt 'P 1 21/c 1' _atom_sites_solution_hydrogens geom _atom_sites_solution_primary direct _audit_creation_method ; Olex2 1.2 (compiled 2015.01.26 svn.r3150 for OlexSys, GUI svn.r4998) ; _cell_angle_alpha 90 _cell_angle_beta 117.197(18) _cell_angle_gamma 90 _cell_formula_units_Z 4 _cell_length_a 14.576(2) _cell_length_b 11.0945(9) _cell_length_c 15.700(2) _cell_measurement_reflns_used 3865 _cell_measurement_temperature 114(7) _cell_measurement_theta_max 28.9790 _cell_measurement_theta_min 2.8820 _cell_volume 2258.2(6) _computing_cell_refinement ; CrysAlisPro (Rigaku OD, 2022) ; _computing_data_collection ; CrysAlisPro (Rigaku OD, 2022) ; _computing_data_reduction ; CrysAlisPro (Rigaku OD, 2022) ; _computing_molecular_graphics ; Olex2 (Dolomanov et al., 2009) ; _computing_publication_material ; Olex2 (Dolomanov et al., 2009) ; _computing_structure_refinement ; ShelXL (Sheldrick, 2015) ; _computing_structure_solution ; ShelXS (Sheldrick, 2008) ; _diffrn_ambient_temperature 114(7) _diffrn_detector_area_resol_mean 15.9631 _diffrn_measured_fraction_theta_full 0.999 _diffrn_measured_fraction_theta_max 0.999 _diffrn_measurement_device_type 'SuperNova, Single source at offset, Eos' _diffrn_measurement_method '\w scans' _diffrn_radiation_monochromator mirror _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_av_R_equivalents 0.0278 _diffrn_reflns_av_unetI/netI 0.0484 _diffrn_reflns_limit_h_max 18 _diffrn_reflns_limit_h_min -9 _diffrn_reflns_limit_k_max 13 _diffrn_reflns_limit_k_min -12 _diffrn_reflns_limit_l_max 19 _diffrn_reflns_limit_l_min -19 _diffrn_reflns_number 8975 _diffrn_reflns_theta_full 25.242 _diffrn_reflns_theta_max 26.371 _diffrn_reflns_theta_min 2.423 _diffrn_source 'SuperNova (Mo) X-ray Source' _exptl_absorpt_coefficient_mu 6.363 _exptl_absorpt_correction_T_max 1.00000 _exptl_absorpt_correction_T_min 0.57936 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details ; (CrysAlisPro; Rigaku OD, 2022) ; _exptl_crystal_colour colourless _exptl_crystal_density_diffrn 1.833 _exptl_crystal_description block _exptl_crystal_F_000 1216 _exptl_crystal_size_max 0.27 _exptl_crystal_size_mid 0.2 _exptl_crystal_size_min 0.16 _refine_diff_density_max 0.846 _refine_diff_density_min -1.073 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.039 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 292 _refine_ls_number_reflns 4603 _refine_ls_number_restraints 288 _refine_ls_restrained_S_all 1.016 _refine_ls_R_factor_all 0.0395 _refine_ls_R_factor_gt 0.0296 _refine_ls_shift/su_max 0.001 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0148P)^2^] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.0515 _refine_ls_wR_factor_ref 0.0556 _reflns_number_gt 3885 _reflns_number_total 4603 _reflns_threshold_expression 'I > 2\s(I)' _iucr_refine_instructions_details ; chi36.res created by SHELXL-2014/7 TITL chi36 in P21/c #14 REM reset to P21/c #14 CELL 0.71073 14.575565 11.094495 15.699614 90 117.1969 90 ZERR 4 0.002008 0.000931 0.002162 0 0.0177 0 LATT 1 SYMM -X,0.5+Y,0.5-Z SFAC C H Cl N O Pt UNIT 96 104 4 4 16 4 RIGU L.S. 20 PLAN 5 TEMP -178 BOND $H CONF ACTA BOND fmap 2 acta SHEL 900 0.8 REM REM REM WGHT 0.014800 FVAR 2.39925 0.92826 PART 2 PT1A 6 0.489460 0.893963 0.131466 21.00000 0.03098 0.02179 = 0.02215 -0.00014 0.01123 -0.00439 PART 0 PART 1 PT1B 6 0.476347 0.860000 0.146930 -21.00000 0.02648 0.02470 = 0.03426 -0.00840 0.01466 -0.00413 PART 0 CL2 3 0.381946 0.977950 0.188733 11.00000 0.04308 0.03418 = 0.03363 -0.00522 0.01991 -0.00156 N3 4 0.614013 0.976877 0.253074 11.00000 0.04290 0.02854 = 0.03200 0.00049 0.01728 -0.00232 C4 1 0.634265 1.090127 0.243085 11.00000 0.04109 0.02210 = 0.03704 -0.00067 0.01925 0.00053 AFIX 43 H4 2 0.602812 1.123141 0.180315 11.00000 -1.20000 AFIX 0 C5 1 0.698760 1.165477 0.318191 11.00000 0.04571 0.02429 = 0.04081 -0.00569 0.02746 -0.00645 AFIX 43 H5 2 0.709989 1.247096 0.307181 11.00000 -1.20000 AFIX 0 C6 1 0.745250 1.116268 0.408728 11.00000 0.03904 0.03340 = 0.04044 -0.01271 0.02370 -0.00843 AFIX 43 H6 2 0.788665 1.164474 0.462019 11.00000 -1.20000 AFIX 0 C7 1 0.728192 0.993764 0.422173 11.00000 0.02755 0.02433 = 0.02780 -0.00296 0.01477 -0.00064 C8 1 0.776352 0.937522 0.512842 11.00000 0.03598 0.04207 = 0.03444 0.00109 0.01245 0.00188 AFIX 43 H8 2 0.821093 0.983324 0.567167 11.00000 -1.20000 AFIX 0 C9 1 0.760140 0.820067 0.523918 11.00000 0.04568 0.04411 = 0.03632 0.00487 0.01433 0.00620 AFIX 43 H9 2 0.794385 0.782665 0.584960 11.00000 -1.20000 AFIX 0 C10 1 0.691693 0.754199 0.443500 11.00000 0.04409 0.03464 = 0.03395 0.00680 0.01936 0.00030 AFIX 43 H10 2 0.679784 0.671783 0.451595 11.00000 -1.20000 AFIX 0 C11 1 0.641654 0.803453 0.354389 11.00000 0.03862 0.02988 = 0.03103 0.00056 0.01725 -0.00442 AFIX 43 H11 2 0.594968 0.756544 0.301769 11.00000 -1.20000 AFIX 0 C12 1 0.660426 0.926397 0.341340 11.00000 0.02652 0.03456 = 0.02780 0.00026 0.01539 0.00282 C13 1 0.581712 0.873631 0.062322 11.00000 0.03192 0.04054 = 0.02896 -0.00608 0.01088 0.00025 PART 2 AFIX 23 H13C 2 0.546236 0.879678 -0.008409 21.00000 -1.20000 H13D 2 0.649595 0.914473 0.092226 21.00000 -1.20000 AFIX 23 PART 0 PART 1 H13A 2 0.545215 0.882003 -0.008239 -21.00000 -1.20000 H13B 2 0.647624 0.918380 0.094028 -21.00000 -1.20000 AFIX 0 PART 0 C14 1 0.575852 0.762763 0.101039 11.00000 0.02940 0.03469 = 0.03005 -0.00461 0.00964 0.00536 PART 2 AFIX 13 H14A 2 0.640640 0.734951 0.156968 21.00000 -1.20000 AFIX 13 PART 0 PART 1 H14 2 0.642287 0.733697 0.154244 -21.00000 -1.20000 AFIX 0 PART 0 C15 1 0.503463 0.663378 0.039695 11.00000 0.04277 0.02563 = 0.03265 -0.00035 0.01489 -0.00036 AFIX 23 H15A 2 0.529816 0.628769 -0.003018 11.00000 -1.20000 H15B 2 0.500494 0.598158 0.081403 11.00000 -1.20000 AFIX 0 C16 1 0.396833 0.714411 -0.019507 11.00000 0.03179 0.02328 = 0.03009 -0.00127 0.01518 -0.00517 C17 1 0.322553 0.656432 -0.100551 11.00000 0.03875 0.02518 = 0.03152 -0.00439 0.02082 -0.00770 AFIX 43 H17 2 0.340049 0.585136 -0.123366 11.00000 -1.20000 AFIX 0 C18 1 0.223562 0.702252 -0.147839 11.00000 0.03559 0.03722 = 0.02747 -0.00794 0.01505 -0.01554 C19 1 0.200623 0.810210 -0.116278 11.00000 0.02810 0.04375 = 0.02593 -0.00272 0.01575 -0.00480 C20 1 0.274269 0.868060 -0.035818 11.00000 0.03490 0.03063 = 0.02654 -0.00355 0.01765 -0.00169 AFIX 43 H20 2 0.256936 0.941204 -0.015155 11.00000 -1.20000 AFIX 0 C21 1 0.373729 0.820706 0.015572 11.00000 0.03113 0.02595 = 0.02707 0.00363 0.01584 -0.00496 O22 5 0.142472 0.647599 -0.224393 11.00000 0.03535 0.05005 = 0.03590 -0.01665 0.01389 -0.01500 C23 1 0.163183 0.539299 -0.261506 11.00000 0.05040 0.04843 = 0.03847 -0.01654 0.02257 -0.02240 AFIX 137 H23A 2 0.098943 0.508514 -0.313448 11.00000 -1.50000 H23B 2 0.192140 0.478959 -0.210405 11.00000 -1.50000 H23C 2 0.212695 0.556025 -0.286161 11.00000 -1.50000 AFIX 0 O24 5 0.100448 0.856105 -0.160523 11.00000 0.02672 0.06321 = 0.03236 -0.00756 0.01336 -0.00063 C25 1 0.068136 0.899580 -0.255398 11.00000 0.02898 0.05501 = 0.02894 -0.00934 0.00680 0.00479 AFIX 23 H25A 2 -0.007823 0.892760 -0.291982 11.00000 -1.20000 H25B 2 0.098844 0.848605 -0.287488 11.00000 -1.20000 AFIX 0 C26 1 0.098900 1.027588 -0.256694 11.00000 0.02564 0.05146 = 0.03291 -0.00978 0.00482 0.00908 O27 5 0.149588 1.089607 -0.188944 11.00000 0.05346 0.04733 = 0.03687 -0.01133 -0.00321 0.00493 O28 5 0.059158 1.064683 -0.348174 11.00000 0.03870 0.04839 = 0.03403 -0.00790 0.00677 0.00615 C29 1 0.079849 1.188776 -0.364300 11.00000 0.04334 0.04546 = 0.04794 -0.00236 0.01124 0.01466 AFIX 23 H29A 2 0.155066 1.202309 -0.337600 11.00000 -1.20000 H29B 2 0.052135 1.245189 -0.332891 11.00000 -1.20000 AFIX 0 C30 1 0.028031 1.208660 -0.470254 11.00000 0.05468 0.06949 = 0.04557 0.00352 0.02371 0.01937 AFIX 23 H30A 2 -0.046320 1.189780 -0.496426 11.00000 -1.20000 H30B 2 0.057981 1.153300 -0.500373 11.00000 -1.20000 AFIX 0 C31 1 0.040654 1.338293 -0.495264 11.00000 0.11820 0.06634 = 0.05720 0.00968 0.03648 0.03799 AFIX 137 H31A 2 0.018338 1.344562 -0.564208 11.00000 -1.50000 H31B 2 0.113282 1.361948 -0.459944 11.00000 -1.50000 H31C 2 -0.001541 1.391730 -0.477722 11.00000 -1.50000 AFIX 0 HKLF 4 REM chi36 in P21/c #14 REM R1 = 0.0296 for 3885 Fo > 4sig(Fo) and 0.0395 for all 4603 data REM 292 parameters refined using 288 restraints END WGHT 0.0148 0.0000 REM Highest difference peak 0.846, deepest hole -1.073, 1-sigma level 0.115 Q1 1 0.5011 0.9559 0.1707 11.00000 0.05 0.85 Q2 1 0.4603 0.8351 0.0815 11.00000 0.05 0.75 Q3 1 0.5963 0.8756 0.2909 11.00000 0.05 0.73 Q4 1 0.4574 0.9502 0.0917 11.00000 0.05 0.71 Q5 1 0.5560 0.8925 0.1388 11.00000 0.05 0.59 REM The information below was added by Olex2. REM REM R1 = 0.0296 for 3885 Fo > 4sig(Fo) and 0.0395 for all 9990 data REM n/a parameters refined using n/a restraints REM Highest difference peak 0.85, deepest hole -1.07 REM Mean Shift 0, Max Shift -0.001. REM +++ Tabular Listing of Refinement Information +++ REM R1_all = 0.0395 REM R1_gt = 0.0296 REM wR_ref = 0.0556 REM GOOF = 1.039 REM Shift_max = -0.001 REM Shift_mean = 0 REM Reflections_all = 9990 REM Reflections_gt = 3885 REM Parameters = n/a REM Hole = -1.07 REM Peak = 0.85 REM Flack = n/a ; _cod_data_source_file pk2707.cif _cod_data_source_block III _cod_original_cell_volume 2258.1(6) _cod_database_code 2023136 _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y-1/2, z-1/2' loop_ _atom_site_type_symbol _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group Pt Pt1A 0.48946(7) 0.89396(12) 0.13147(5) 0.02532(15) Uani d 0.928(7) A 2 Pt Pt1B 0.4763(6) 0.8600(18) 0.1469(11) 0.028(2) Uani d 0.072(7) A 1 Cl Cl2 0.38195(9) 0.97795(9) 0.18873(8) 0.0360(3) Uani d 1 . . N N3 0.6140(3) 0.9769(3) 0.2531(2) 0.0344(9) Uani d 1 . . C C4 0.6343(3) 1.0901(3) 0.2431(3) 0.0329(10) Uani d 1 . . H H4 0.6028 1.1231 0.1803 0.039 Uiso calc 1 . . C C5 0.6988(3) 1.1655(4) 0.3182(3) 0.0340(10) Uani d 1 . . H H5 0.7100 1.2471 0.3072 0.041 Uiso calc 1 . . C C6 0.7452(3) 1.1163(4) 0.4087(3) 0.0355(11) Uani d 1 . . H H6 0.7887 1.1645 0.4620 0.043 Uiso calc 1 . . C C7 0.7282(3) 0.9938(3) 0.4222(3) 0.0257(9) Uani d 1 . . C C8 0.7764(3) 0.9375(4) 0.5128(3) 0.0389(11) Uani d 1 . . H H8 0.8211 0.9833 0.5672 0.047 Uiso calc 1 . . C C9 0.7601(4) 0.8201(4) 0.5239(3) 0.0437(12) Uani d 1 . . H H9 0.7944 0.7827 0.5850 0.052 Uiso calc 1 . . C C10 0.6917(3) 0.7542(4) 0.4435(3) 0.0370(11) Uani d 1 . . H H10 0.6798 0.6718 0.4516 0.044 Uiso calc 1 . . C C11 0.6417(3) 0.8035(4) 0.3544(3) 0.0327(10) Uani d 1 . . H H11 0.5950 0.7565 0.3018 0.039 Uiso calc 1 . . C C12 0.6604(3) 0.9264(4) 0.3413(3) 0.0285(9) Uani d 1 . . C C13 0.5817(3) 0.8736(4) 0.0623(3) 0.0350(11) Uani d 1 . . H H13C 0.5462 0.8797 -0.0084 0.042 Uiso calc 0.928(7) A 2 H H13D 0.6496 0.9145 0.0922 0.042 Uiso calc 0.928(7) A 2 H H13A 0.5452 0.8820 -0.0082 0.042 Uiso calc 0.072(7) A 1 H H13B 0.6476 0.9184 0.0940 0.042 Uiso calc 0.072(7) A 1 C C14 0.5759(3) 0.7628(4) 0.1010(3) 0.0329(10) Uani d 1 . . H H14A 0.6406 0.7350 0.1570 0.039 Uiso calc 0.928(7) A 2 H H14 0.6423 0.7337 0.1542 0.039 Uiso calc 0.072(7) A 1 C C15 0.5035(3) 0.6634(4) 0.0397(3) 0.0346(10) Uani d 1 . . H H15A 0.5298 0.6288 -0.0030 0.042 Uiso calc 1 . . H H15B 0.5005 0.5982 0.0814 0.042 Uiso calc 1 . . C C16 0.3968(3) 0.7144(3) -0.0195(3) 0.0280(9) Uani d 1 . . C C17 0.3226(3) 0.6564(4) -0.1006(3) 0.0300(10) Uani d 1 . . H H17 0.3400 0.5851 -0.1234 0.036 Uiso calc 1 . . C C18 0.2236(3) 0.7023(4) -0.1478(3) 0.0332(10) Uani d 1 . . C C19 0.2006(3) 0.8102(4) -0.1163(3) 0.0313(10) Uani d 1 . . C C20 0.2743(3) 0.8681(4) -0.0358(3) 0.0293(10) Uani d 1 . . H H20 0.2569 0.9412 -0.0152 0.035 Uiso calc 1 . . C C21 0.3737(3) 0.8207(4) 0.0156(3) 0.0271(9) Uani d 1 . . O O22 0.1425(2) 0.6476(3) -0.2244(2) 0.0414(8) Uani d 1 . . C C23 0.1632(4) 0.5393(4) -0.2615(3) 0.0449(13) Uani d 1 . . H H23A 0.0989 0.5085 -0.3134 0.067 Uiso calc 1 . . H H23B 0.1921 0.4790 -0.2104 0.067 Uiso calc 1 . . H H23C 0.2127 0.5560 -0.2862 0.067 Uiso calc 1 . . O O24 0.1004(2) 0.8561(3) -0.1605(2) 0.0408(8) Uani d 1 . . C C25 0.0681(3) 0.8996(4) -0.2554(3) 0.0401(11) Uani d 1 . . H H25A -0.0078 0.8928 -0.2920 0.048 Uiso calc 1 . . H H25B 0.0988 0.8486 -0.2875 0.048 Uiso calc 1 . . C C26 0.0989(3) 1.0276(4) -0.2567(3) 0.0400(11) Uani d 1 . . O O27 0.1496(3) 1.0896(3) -0.1889(2) 0.0551(10) Uani d 1 . . O O28 0.0592(2) 1.0647(3) -0.3482(2) 0.0442(8) Uani d 1 . . C C29 0.0798(4) 1.1888(4) -0.3643(3) 0.0493(13) Uani d 1 . . H H29A 0.1551 1.2023 -0.3376 0.059 Uiso calc 1 . . H H29B 0.0521 1.2452 -0.3329 0.059 Uiso calc 1 . . C C30 0.0280(4) 1.2087(5) -0.4703(4) 0.0563(14) Uani d 1 . . H H30A -0.0463 1.1898 -0.4964 0.068 Uiso calc 1 . . H H30B 0.0580 1.1533 -0.5004 0.068 Uiso calc 1 . . C C31 0.0407(5) 1.3383(5) -0.4953(4) 0.082(2) Uani d 1 . . H H31A 0.0183 1.3446 -0.5642 0.123 Uiso calc 1 . . H H31B 0.1133 1.3619 -0.4599 0.123 Uiso calc 1 . . H H31C -0.0015 1.3917 -0.4777 0.123 Uiso calc 1 . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Pt1A 0.03098(18) 0.0218(3) 0.02215(15) -0.00439(19) 0.01123(11) -0.00014(15) Pt1B 0.0265(18) 0.025(4) 0.034(3) -0.0041(19) 0.0147(16) -0.008(3) Cl2 0.0431(7) 0.0342(6) 0.0336(6) -0.0016(5) 0.0199(5) -0.0052(5) N3 0.043(2) 0.0285(18) 0.0320(19) -0.0023(17) 0.0173(17) 0.0005(15) C4 0.041(3) 0.022(2) 0.037(2) 0.001(2) 0.019(2) -0.0007(18) C5 0.046(3) 0.024(2) 0.041(2) -0.006(2) 0.027(2) -0.0057(19) C6 0.039(3) 0.033(2) 0.040(2) -0.008(2) 0.024(2) -0.0127(19) C7 0.028(2) 0.024(2) 0.028(2) -0.0006(18) 0.0148(18) -0.0030(17) C8 0.036(3) 0.042(2) 0.034(2) 0.002(2) 0.012(2) 0.001(2) C9 0.046(3) 0.044(3) 0.036(3) 0.006(2) 0.014(2) 0.005(2) C10 0.044(3) 0.035(2) 0.034(2) 0.000(2) 0.019(2) 0.0068(19) C11 0.039(3) 0.030(2) 0.031(2) -0.004(2) 0.017(2) 0.0006(18) C12 0.027(2) 0.035(2) 0.028(2) 0.0028(18) 0.0154(18) 0.0003(17) C13 0.032(2) 0.041(2) 0.029(2) 0.000(2) 0.011(2) -0.006(2) C14 0.029(2) 0.035(2) 0.030(2) 0.0054(19) 0.010(2) -0.0046(19) C15 0.043(3) 0.026(2) 0.033(2) 0.000(2) 0.015(2) -0.0003(19) C16 0.032(2) 0.023(2) 0.030(2) -0.0052(18) 0.0152(18) -0.0013(17) C17 0.039(2) 0.025(2) 0.032(2) -0.0077(19) 0.0208(19) -0.0044(18) C18 0.036(2) 0.037(2) 0.027(2) -0.0155(19) 0.0151(19) -0.0079(19) C19 0.028(2) 0.044(2) 0.026(2) -0.0048(19) 0.0158(18) -0.0027(19) C20 0.035(2) 0.031(2) 0.027(2) -0.0017(19) 0.0176(18) -0.0036(18) C21 0.031(2) 0.026(2) 0.027(2) -0.0050(18) 0.0158(17) 0.0036(17) O22 0.0353(18) 0.0500(18) 0.0359(18) -0.0150(16) 0.0139(15) -0.0166(15) C23 0.050(3) 0.048(3) 0.038(3) -0.022(3) 0.023(3) -0.017(2) O24 0.0267(16) 0.063(2) 0.0324(17) -0.0006(15) 0.0134(14) -0.0076(16) C25 0.029(2) 0.055(3) 0.029(2) 0.005(2) 0.007(2) -0.009(2) C26 0.026(2) 0.051(3) 0.033(2) 0.009(2) 0.005(2) -0.010(2) O27 0.053(2) 0.047(2) 0.0369(19) 0.0049(18) -0.0032(18) -0.0113(16) O28 0.0387(19) 0.0484(19) 0.0340(18) 0.0061(16) 0.0068(15) -0.0079(15) C29 0.043(3) 0.045(3) 0.048(3) 0.015(2) 0.011(2) -0.002(2) C30 0.055(3) 0.069(3) 0.046(3) 0.019(3) 0.024(3) 0.004(3) C31 0.118(6) 0.066(4) 0.057(4) 0.038(4) 0.036(4) 0.010(3) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0033 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Cl Cl 0.1484 0.1585 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0061 0.0033 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0106 0.0060 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Pt Pt -1.7033 8.3905 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag N3 Pt1A Cl2 . . 85.99(10) ? C13 Pt1A Cl2 . . 161.77(14) ? C13 Pt1A N3 . . 91.42(16) ? C13 Pt1A C14 . . 38.62(14) ? C14 Pt1A Cl2 . . 159.56(15) ? C14 Pt1A N3 . . 98.43(15) ? C21 Pt1A Cl2 . . 94.43(13) ? C21 Pt1A N3 . . 178.23(17) ? C21 Pt1A C13 . . 87.65(17) ? C21 Pt1A C14 . . 81.77(16) ? Cl2 Pt1B N3 . . 84.7(3) ? Cl2 Pt1B C13 . . 139.1(12) ? N3 Pt1B C13 . . 78.8(6) ? C14 Pt1B Cl2 . . 173.3(14) ? C14 Pt1B N3 . . 91.5(4) ? C14 Pt1B C13 . . 34.4(3) ? C21 Pt1B Cl2 . . 99.5(3) ? C21 Pt1B N3 . . 150.2(15) ? C21 Pt1B C13 . . 79.0(6) ? C21 Pt1B C14 . . 81.1(4) ? C4 N3 Pt1A . . 116.6(3) ? C4 N3 Pt1B . . 127.8(7) ? C4 N3 C12 . . 118.8(4) ? C12 N3 Pt1A . . 123.8(3) ? C12 N3 Pt1B . . 111.5(7) ? N3 C4 H4 . . 117.6 ? N3 C4 C5 . . 124.8(4) ? C5 C4 H4 . . 117.6 ? C4 C5 H5 . . 121.4 ? C6 C5 C4 . . 117.2(4) ? C6 C5 H5 . . 121.4 ? C5 C6 H6 . . 120.1 ? C5 C6 C7 . . 119.8(4) ? C7 C6 H6 . . 120.1 ? C8 C7 C6 . . 122.3(4) ? C8 C7 C12 . . 119.5(4) ? C12 C7 C6 . . 118.2(4) ? C7 C8 H8 . . 119.3 ? C9 C8 C7 . . 121.4(4) ? C9 C8 H8 . . 119.3 ? C8 C9 H9 . . 120.6 ? C8 C9 C10 . . 118.7(4) ? C10 C9 H9 . . 120.6 ? C9 C10 H10 . . 118.6 ? C11 C10 C9 . . 122.8(4) ? C11 C10 H10 . . 118.6 ? C10 C11 H11 . . 120.5 ? C10 C11 C12 . . 119.0(4) ? C12 C11 H11 . . 120.5 ? N3 C12 C7 . . 121.1(4) ? N3 C12 C11 . . 120.3(4) ? C7 C12 C11 . . 118.6(4) ? Pt1A C13 H13C . . 116.4 ? Pt1A C13 H13D . . 116.4 ? Pt1B C13 H13A . . 117.6 ? Pt1B C13 H13B . . 117.6 ? H13C C13 H13D . . 113.4 ? H13A C13 H13B . . 114.7 ? C14 C13 Pt1A . . 71.7(3) ? C14 C13 Pt1B . . 62.0(5) ? C14 C13 H13C . . 116.4 ? C14 C13 H13D . . 116.4 ? C14 C13 H13A . . 117.6 ? C14 C13 H13B . . 117.6 ? Pt1A C14 H14A . . 115.7 ? Pt1B C14 H14 . . 114.9 ? C13 C14 Pt1A . . 69.7(2) ? C13 C14 Pt1B . . 83.7(8) ? C13 C14 H14A . . 115.7 ? C13 C14 H14 . . 114.9 ? C13 C14 C15 . . 121.7(4) ? C15 C14 Pt1A . . 109.2(3) ? C15 C14 Pt1B . . 101.2(5) ? C15 C14 H14A . . 115.7 ? C15 C14 H14 . . 114.9 ? C14 C15 H15A . . 109.7 ? C14 C15 H15B . . 109.7 ? H15A C15 H15B . . 108.2 ? C16 C15 C14 . . 109.7(3) ? C16 C15 H15A . . 109.7 ? C16 C15 H15B . . 109.7 ? C17 C16 C15 . . 122.7(4) ? C17 C16 C21 . . 121.3(4) ? C21 C16 C15 . . 115.9(4) ? C16 C17 H17 . . 119.8 ? C18 C17 C16 . . 120.3(4) ? C18 C17 H17 . . 119.8 ? C17 C18 C19 . . 119.1(4) ? O22 C18 C17 . . 125.0(4) ? O22 C18 C19 . . 115.9(4) ? C18 C19 O24 . . 120.2(4) ? C20 C19 C18 . . 120.7(4) ? C20 C19 O24 . . 118.9(4) ? C19 C20 H20 . . 119.4 ? C19 C20 C21 . . 121.2(4) ? C21 C20 H20 . . 119.4 ? C16 C21 Pt1A . . 116.3(3) ? C16 C21 Pt1B . . 113.2(4) ? C20 C21 Pt1A . . 126.3(3) ? C20 C21 Pt1B . . 127.8(4) ? C20 C21 C16 . . 117.3(4) ? C18 O22 C23 . . 117.9(4) ? O22 C23 H23A . . 109.5 ? O22 C23 H23B . . 109.5 ? O22 C23 H23C . . 109.5 ? H23A C23 H23B . . 109.5 ? H23A C23 H23C . . 109.5 ? H23B C23 H23C . . 109.5 ? C19 O24 C25 . . 114.5(3) ? O24 C25 H25A . . 109.2 ? O24 C25 H25B . . 109.2 ? O24 C25 C26 . . 112.2(4) ? H25A C25 H25B . . 107.9 ? C26 C25 H25A . . 109.2 ? C26 C25 H25B . . 109.2 ? O27 C26 C25 . . 127.0(5) ? O27 C26 O28 . . 124.3(5) ? O28 C26 C25 . . 108.7(4) ? C26 O28 C29 . . 116.9(4) ? O28 C29 H29A . . 110.3 ? O28 C29 H29B . . 110.3 ? O28 C29 C30 . . 107.1(4) ? H29A C29 H29B . . 108.6 ? C30 C29 H29A . . 110.3 ? C30 C29 H29B . . 110.3 ? C29 C30 H30A . . 109.3 ? C29 C30 H30B . . 109.3 ? C29 C30 C31 . . 111.5(4) ? H30A C30 H30B . . 108.0 ? C31 C30 H30A . . 109.3 ? C31 C30 H30B . . 109.3 ? C30 C31 H31A . . 109.5 ? C30 C31 H31B . . 109.5 ? C30 C31 H31C . . 109.5 ? H31A C31 H31B . . 109.5 ? H31A C31 H31C . . 109.5 ? H31B C31 H31C . . 109.5 ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag Pt1A Cl2 . 2.3281(14) ? Pt1A N3 . 2.149(4) ? Pt1A C13 . 2.091(4) ? Pt1A C14 . 2.117(4) ? Pt1A C21 . 2.003(4) ? Pt1B Cl2 . 2.205(6) ? Pt1B N3 . 2.330(11) ? Pt1B C13 . 2.45(2) ? Pt1B C14 . 2.178(9) ? Pt1B C21 . 1.965(9) ? N3 C4 . 1.316(5) ? N3 C12 . 1.354(5) ? C4 H4 . 0.9500 ? C4 C5 . 1.400(6) ? C5 H5 . 0.9500 ? C5 C6 . 1.377(6) ? C6 H6 . 0.9500 ? C6 C7 . 1.415(5) ? C7 C8 . 1.412(5) ? C7 C12 . 1.414(5) ? C8 H8 . 0.9500 ? C8 C9 . 1.350(6) ? C9 H9 . 0.9500 ? C9 C10 . 1.404(6) ? C10 H10 . 0.9500 ? C10 C11 . 1.362(5) ? C11 H11 . 0.9500 ? C11 C12 . 1.424(5) ? C13 H13C . 0.9900 ? C13 H13D . 0.9900 ? C13 H13A . 0.9900 ? C13 H13B . 0.9900 ? C13 C14 . 1.392(5) ? C14 H14A . 1.0000 ? C14 H14 . 1.0000 ? C14 C15 . 1.526(5) ? C15 H15A . 0.9900 ? C15 H15B . 0.9900 ? C15 C16 . 1.510(5) ? C16 C17 . 1.395(5) ? C16 C21 . 1.406(5) ? C17 H17 . 0.9500 ? C17 C18 . 1.383(6) ? C18 C19 . 1.394(6) ? C18 O22 . 1.382(5) ? C19 C20 . 1.386(5) ? C19 O24 . 1.395(5) ? C20 H20 . 0.9500 ? C20 C21 . 1.400(5) ? O22 C23 . 1.427(5) ? C23 H23A . 0.9800 ? C23 H23B . 0.9800 ? C23 H23C . 0.9800 ? O24 C25 . 1.425(5) ? C25 H25A . 0.9900 ? C25 H25B . 0.9900 ? C25 C26 . 1.492(6) ? C26 O27 . 1.197(5) ? C26 O28 . 1.344(5) ? O28 C29 . 1.456(5) ? C29 H29A . 0.9900 ? C29 H29B . 0.9900 ? C29 C30 . 1.496(6) ? C30 H30A . 0.9900 ? C30 H30B . 0.9900 ? C30 C31 . 1.524(7) ? C31 H31A . 0.9800 ? C31 H31B . 0.9800 ? C31 H31C . 0.9800 ? loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_site_symmetry_D _geom_hbond_site_symmetry_H _geom_hbond_site_symmetry_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA _geom_hbond_publ_flag C9 H9 O27 1_555 1_555 2_644 0.95 2.59 3.445(5) 150 y C23 H23C Cl2 1_555 1_555 4_575 0.98 2.70 3.618(6) 157 y C29 H29B O24 1_555 1_555 2_554 0.99 2.50 3.381(7) 148 y C6 H6 Cg1 1_555 1_555 2_655 0.95 2.73 3.269(5) 117 y loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion _geom_torsion_publ_flag Pt1A N3 C4 C5 . . . . 167.9(3) ? Pt1A N3 C12 C7 . . . . -168.1(3) ? Pt1A N3 C12 C11 . . . . 11.9(5) ? Pt1A C13 C14 C15 . . . . 100.5(4) ? Pt1A C14 C15 C16 . . . . 28.6(4) ? Pt1B N3 C4 C5 . . . . 160.7(5) ? Pt1B N3 C12 C7 . . . . -164.3(4) ? Pt1B N3 C12 C11 . . . . 15.7(5) ? Pt1B C13 C14 C15 . . . . 99.3(4) ? Pt1B C14 C15 C16 . . . . 40.6(8) ? N3 C4 C5 C6 . . . . 1.0(7) ? C4 N3 C12 C7 . . . . 1.1(6) ? C4 N3 C12 C11 . . . . -178.9(4) ? C4 C5 C6 C7 . . . . 1.1(6) ? C5 C6 C7 C8 . . . . 178.0(4) ? C5 C6 C7 C12 . . . . -2.0(6) ? C6 C7 C8 C9 . . . . -179.1(4) ? C6 C7 C12 N3 . . . . 0.9(6) ? C6 C7 C12 C11 . . . . -179.1(4) ? C7 C8 C9 C10 . . . . -1.7(7) ? C8 C7 C12 N3 . . . . -179.1(4) ? C8 C7 C12 C11 . . . . 0.9(6) ? C8 C9 C10 C11 . . . . 0.7(7) ? C9 C10 C11 C12 . . . . 1.1(7) ? C10 C11 C12 N3 . . . . 178.1(4) ? C10 C11 C12 C7 . . . . -1.8(6) ? C12 N3 C4 C5 . . . . -2.1(7) ? C12 C7 C8 C9 . . . . 0.9(6) ? C13 C14 C15 C16 . . . . -48.9(5) ? C14 C15 C16 C17 . . . . 161.5(4) ? C14 C15 C16 C21 . . . . -22.8(5) ? C15 C16 C17 C18 . . . . 174.9(4) ? C15 C16 C21 Pt1A . . . . 5.0(5) ? C15 C16 C21 Pt1B . . . . -11.5(9) ? C15 C16 C21 C20 . . . . -177.8(3) ? C16 C17 C18 C19 . . . . 3.2(6) ? C16 C17 C18 O22 . . . . -175.2(4) ? C17 C16 C21 Pt1A . . . . -179.2(3) ? C17 C16 C21 Pt1B . . . . 164.3(9) ? C17 C16 C21 C20 . . . . -2.0(6) ? C17 C18 C19 C20 . . . . -3.2(6) ? C17 C18 C19 O24 . . . . -177.7(4) ? C17 C18 O22 C23 . . . . -3.9(6) ? C18 C19 C20 C21 . . . . 0.5(6) ? C18 C19 O24 C25 . . . . -69.9(5) ? C19 C18 O22 C23 . . . . 177.7(4) ? C19 C20 C21 Pt1A . . . . 178.9(3) ? C19 C20 C21 Pt1B . . . . -162.0(11) ? C19 C20 C21 C16 . . . . 2.0(6) ? C19 O24 C25 C26 . . . . -86.2(4) ? C20 C19 O24 C25 . . . . 115.6(4) ? C21 C16 C17 C18 . . . . -0.6(6) ? O22 C18 C19 C20 . . . . 175.4(4) ? O22 C18 C19 O24 . . . . 0.9(6) ? O24 C19 C20 C21 . . . . 175.1(3) ? O24 C25 C26 O27 . . . . 4.0(7) ? O24 C25 C26 O28 . . . . -175.4(3) ? C25 C26 O28 C29 . . . . 179.3(4) ? C26 O28 C29 C30 . . . . -179.8(4) ? O27 C26 O28 C29 . . . . -0.1(7) ? O28 C29 C30 C31 . . . . 177.4(4) ? loop_ _refln_index_h _refln_index_k _refln_index_l _refln_F_squared_meas _refln_F_squared_sigma 0 0 2 17297.5 724.14 0 0 -2 18751.6 792.22 0 0 3 -40.7221 145.74 0 0 4 212200 4139.28 0 0 -4 202633 3380.2 0 0 -5 88.8814 89.4643 0 0 5 100.129 183.577 0 0 -5 156.295 87.8822 0 0 6 83882.7 2853.84 0 0 -6 81762.3 2115.47 0 0 -6 80497.6 2636.57 0 0 7 -15.3971 260.053 0 0 -7 152.156 163.339 0 0 8 234160 5799.69 0 0 -8 229511 4406.53 0 0 -9 97.6239 136.522 0 0 9 589.594 410.56 0 0 -10 46926.5 1832.89 0 0 10 47772.1 2739.71 0 0 -11 303.115 179.125 0 0 11 -87.6614 335.573 0 0 12 43441.8 2877.18 0 0 -12 46452.1 1925.99 0 0 -13 317.849 243.657 0 0 13 -67.8599 333.589 0 0 14 10896.5 1616.24 0 0 15 1088.3 617.948 0 0 16 29499.3 2805.56 0 0 17 -101.265 440.879 0 1 2 62818.4 1287.02 0 1 2 63262.6 1518.3 0 -1 -2 61606.1 1526.83 0 -1 -2 62773.2 1296.81 0 1 3 219278 3846.2 0 -1 -3 219322 3894.91 0 1 3 215759 3487.49 0 -1 -3 222482 3542 0 -1 -4 334.102 131.17 0 1 -4 292.722 158.911 0 1 4 499.363 176.775 0 -1 -4 529.83 193.925 0 -1 -5 9192.17 831.193 0 1 5 9448.24 815.449 0 -1 -5 9310.02 450.411 0 -1 -5 9763.44 748.583 0 1 -5 9104.13 725.345 0 1 -6 50897.7 1902.29 0 -1 -6 53201.7 1316.45 0 1 6 56848 2257.12 0 -1 6 51709.9 2320.73 0 -1 -6 56954.9 2079.42 0 -1 7 90956.3 3330.67 0 1 -7 85694.1 2617.92 0 -1 -7 88493.1 1932.47 0 1 7 85328.1 3046.07 0 1 -8 502.597 254.849 0 1 8 -100.65 280.565 0 -1 8 18.7893 230.686 0 -1 -8 391.851 145.409 0 1 9 7680.63 1003.68 0 -1 9 6764.05 1043.61 0 -1 -9 8607.1 594.621 0 1 -9 6834.87 755.106 0 1 -10 23796.4 1456.38 0 -1 -10 25742.7 1103.31 0 -1 10 25241.3 1998.89 0 1 10 24356.7 1906.65 0 -1 -11 45598.2 1547.47 0 -1 11 45904.9 2844.28 0 1 -11 41876.4 2011.52 0 1 11 40543.5 2617.6 0 1 -12 1158.99 367.071 0 -1 12 1905.31 641.417 0 1 12 1721.09 571.017 0 -1 -12 877.052 223.14 0 1 -13 17656.5 1339.17 0 -1 13 16578.7 1867.48 0 1 13 16474.8 1855.88 0 -1 14 23137.1 2288.99 0 1 14 24631.6 2380.49 0 -1 15 46259 3394.5 0 1 15 49622.5 3524.82 0 1 16 7560.97 1444.92 0 -1 16 8978.48 1601.2 0 -1 17 70.2546 534.004 0 1 17 1329.13 756.489 0 -2 0 13683.6 494.438 0 2 0 13402.2 500.523 0 2 0 13542.3 712.204 0 2 1 418260 5254.11 0 2 -1 415203 6236.95 0 -2 -1 418820 5253.71 0 2 1 415391 5641.31 0 -2 -2 178516 2776.95 0 2 2 183507 2753.42 0 -2 -2 183390 3325.77 0 2 -2 182817 3636.59 0 2 2 177785 2607.62 0 2 3 122607 2756.65 0 -2 -3 116485 2262.34 0 -2 -3 117914 2740.1 0 2 -3 115502 2946.86 0 2 3 116679 2236.81 0 2 4 410.476 241.348 0 2 -4 352.64 185.998 0 -2 -4 833.883 198.07 0 2 4 406.386 152.443 0 -2 -4 618.498 193.324 0 2 5 349911 6301.92 0 -2 -5 343844 5693.01 0 -2 -5 350957 6382.01 0 2 -5 351169 6312.69 0 2 -6 2586.79 473.042 0 -2 -6 3216.02 457.33 0 2 6 2659.18 523.303 0 2 7 50414.5 2310.39 0 2 -7 50925.9 2185.64 0 2 8 741.692 299.536 0 -2 8 681.074 360.502 0 2 -8 1291.65 362.277 0 2 9 124492 4220.24 0 -2 9 130584 4598.7 0 2 -9 119908 3657.17 0 2 -10 880.986 311.112 0 -2 10 717.116 368.132 0 2 10 691.906 436.3 0 2 11 5549.1 997.841 0 -2 11 6348.56 1089.69 0 2 -11 7655.67 912.834 0 -2 12 112.022 347.983 0 2 12 574.9 352.745 0 2 -12 604.702 233.237 0 2 13 95451.1 4560.69 0 -2 13 104546 4821.32 0 2 -13 99599.2 3580.66 0 -2 14 243.7 453 0 2 -14 312.928 256.088 0 2 14 -705.155 564.542 0 -2 15 -927.658 732.32 0 2 15 -97.9992 492.79 0 -2 16 8995.46 1558.61 0 2 16 8006.56 1613.02 0 2 17 34933.6 3271.75 0 -2 17 33781.8 3176.61 0 3 0 42.9124 129.387 0 -3 0 194.503 92.5899 0 -3 -1 17138.8 783.757 0 3 -1 16574.1 1013.06 0 3 1 17055.3 682.384 0 3 -1 18108.8 669.204 0 3 1 17305.8 903.333 0 3 2 404106 5368.74 0 3 2 388368 5688.03 0 -3 -2 396025 5390.68 0 3 -2 395233 6794.94 0 3 -3 2427.78 451.269 0 3 3 2981.75 318.342 0 -3 -3 3396.09 470.88 0 3 3 2866.72 263.977 0 -3 -3 3494.96 335.199 0 -3 -4 5900.44 626.358 0 3 4 4910.57 450.313 0 3 -4 5499.33 696.07 0 -3 -4 4913.48 451.423 0 -3 -5 55102.3 1781.11 0 3 5 54168.6 1733.81 0 3 -5 56823.7 2332.25 0 3 5 61322.7 2307.68 0 3 6 117441 3523.45 0 3 6 116444 2906.68 0 3 -6 113092 3550.28 0 -3 -6 118375 2974.06 0 3 -7 54661.3 2430.07 0 3 7 51826.7 2417.54 0 3 -8 14525.5 1276.53 0 3 8 14452.4 1340.85 0 3 9 2279.88 629.922 0 -3 9 711.976 632.942 0 3 -9 2217.83 538.075 0 -3 10 83008.5 3919.6 0 3 10 85608.8 3716.94 0 3 -10 84541.4 3273.66 0 -3 11 20791.3 1974.81 0 3 -11 17809.8 1505.95 0 3 -12 11154.2 1217.1 0 -3 12 13033.1 1628.02 0 3 12 13041 1571.99 0 -3 13 2469.95 732.09 0 3 13 1802.02 670.825 0 3 -13 1291.72 463.411 0 3 14 57160.3 3669.14 0 3 -14 53530 2793.43 0 -3 14 51491 3527.12 0 -3 15 9249.29 1586.11 0 3 15 11333.8 1724.6 0 -3 16 17791.6 2246.74 0 3 16 19433.3 2319.94 0 -3 17 -98.6559 517.217 0 3 17 930.253 875.105 0 -4 0 341832 5059.31 0 4 0 341981 6173.48 0 4 -1 89887.5 2837.95 0 -4 -1 91955.1 2155.27 0 4 1 90800.1 2554.05 0 4 1 90943.7 1983.81 0 4 2 828.647 185.124 0 4 2 481.785 176.606 0 4 -2 837.268 301.95 0 -4 -3 5748.85 455.289 0 4 3 5235.57 464.086 0 4 3 5713.57 462.794 0 4 -3 6127.89 805.773 0 -4 -3 6678.69 696.512 0 4 4 204166 3280.87 0 -4 -4 201733 3670.36 0 4 4 200406 3613.31 0 4 -4 208855 5055.05 0 4 5 56427.4 1795.85 0 -4 -5 57708.5 1808.23 0 4 -5 57722 2593.52 0 4 -6 18691.3 1501.91 0 -4 -6 19993 1126.36 0 4 6 19985.3 1092.53 0 4 7 686.445 272.068 0 4 -7 857.676 385.897 0 -4 -7 402.159 181.858 0 4 8 141608 4477.65 0 4 -8 139971 4470 0 4 -9 7085.05 963.75 0 4 9 7969.36 1063.53 0 4 -10 25738.2 1877.39 0 4 10 26132.5 2022.02 0 -4 11 1021.04 569.485 0 4 -11 1418.4 450.626 0 -4 12 56019.3 3508.97 0 4 -12 56332.1 2909.76 0 4 12 56640.9 3343.15 0 4 -13 9757.1 1249.27 0 4 13 13275 1697.19 0 -4 13 13601.7 1762.07 0 4 -14 17101.3 1642.8 0 -4 14 21108.3 2295.22 0 4 14 19613.6 2169.34 0 4 -15 5482.53 962.939 0 4 15 5927.37 1340.37 0 -4 15 4404.43 1042.79 0 4 16 9902.92 1660.5 0 -4 16 6845.34 1427.13 0 -4 17 7120.74 1527.06 0 5 0 188.219 212.667 0 -5 0 142.395 105.883 0 5 -1 196874 3505.42 0 5 -1 191197 4754.56 0 5 1 189149 4429.84 0 5 1 190523 3563.25 0 -5 -1 201899 3802.58 0 5 2 6486.37 670.022 0 5 2 7420.57 553.028 0 -5 -2 6882.3 652.332 0 5 -2 7876.56 918.517 0 5 -2 7860.25 554.413 0 5 3 114563 2508.81 0 5 3 114859 2860 0 5 -3 112953 3754.19 0 5 4 5253.39 487.998 0 -5 -4 4804.44 475.802 0 5 -4 5354.78 813.137 0 5 4 4838.51 469.119 0 -5 -5 56592.4 1818.63 0 5 -5 63271 2851.34 0 5 5 56804.8 1832.67 0 -5 -6 8840.51 748.501 0 5 -6 8906.97 1097.79 0 5 6 9570.76 769.702 0 5 7 139672 3400.59 0 -5 -7 128676 3378.3 0 5 -7 133759 4494.78 0 5 -8 14049.5 1458.44 0 5 -9 10593 1247.88 0 5 -10 2996.02 703.47 0 5 -11 117434 4465.89 0 -5 12 6064.51 1265.99 0 5 -12 6109.61 1011.92 0 5 -13 2054.69 578.835 0 -5 13 1427.33 474.77 0 5 -14 885.691 433.39 0 -5 14 323.085 427.697 0 5 -15 38243.9 2621.93 0 -5 15 39013.2 3293.17 0 -5 16 562.062 514.805 0 -5 17 -433.149 868.945 0 -6 0 24190.2 1173.7 0 6 0 22945.4 1563.25 0 6 1 5686.77 538.823 0 -6 -1 7923.28 674.896 0 6 1 5602.42 726.654 0 6 -1 5454.62 798.282 0 -6 -2 2295.39 411.213 0 6 -2 1662.42 478.121 0 6 2 1352.91 369.582 0 6 2 1398.51 247.678 0 6 -2 1529.77 253.773 0 6 3 59588.5 1817.71 0 6 3 56491.9 2148.79 0 -6 -3 58989.3 2252.62 0 6 -3 55749.2 2727.86 0 6 -3 59751.8 1834.58 0 6 -4 91535 3610.24 0 6 4 84209.2 2295.67 0 6 4 87927 2522.27 0 6 5 73787.3 2121.21 0 -6 -5 70749.1 2129.37 0 6 -5 73819.4 3307.66 0 -6 -6 869.188 251.418 0 6 6 823.808 266.265 0 6 -6 1052.17 471.759 0 6 -7 32019.6 2276.42 0 -6 -7 28705.7 1472.06 0 6 7 32948.6 1538.14 0 6 8 49731.7 2029.28 0 6 -8 43744.8 2695.22 0 6 -9 35865.1 2447.66 0 6 -10 8296.86 1211.88 0 6 -11 9545.84 1305.18 0 6 -12 21415.2 1970.82 0 -6 13 45748.7 3576.01 0 6 -13 52785.5 3140.35 0 -6 14 7262.25 1448.45 0 6 -14 5734.89 1057.19 0 6 -15 125.341 257.498 0 -6 15 -444.712 476.452 0 6 -16 7318.95 1229.41 0 -6 16 5689.06 1335.56 0 -6 17 8982.57 1766.77 0 7 0 -19.7515 271.618 0 7 1 8537.72 740.563 0 7 1 7899.96 959.306 0 -7 -1 9554.51 794.506 0 7 -1 9011.13 1067.95 0 7 -2 204142 3966.44 0 7 2 198297 5006.92 0 7 -2 204589 5700.76 0 7 2 205118 4088.06 0 -7 -2 200682 4442.92 0 7 3 1502.92 385.961 0 -7 -3 800.972 304.195 0 7 -3 1245.8 260.398 0 7 3 1117.87 250.438 0 7 -3 703.404 374.276 0 -7 -4 695.513 292.274 0 7 -4 1157.25 517.188 0 7 4 1137.44 339.032 0 7 -4 1539.1 301.853 0 7 4 866.08 212.997 0 7 5 6832.48 643.444 0 7 -5 5720.03 1004.71 0 7 5 6446.37 670.042 0 7 -6 229217 6585.32 0 -7 -6 217582 4409.87 0 7 6 213081 4363.17 0 7 7 14239.3 1029.96 0 7 -7 16165.9 1647.76 0 7 -8 3159.32 746.851 0 7 8 4388.51 596.854 0 7 -9 7168.73 1189.34 0 7 -10 71947 3806.63 0 7 -11 216.241 362.584 0 7 -12 24762.8 2256.87 0 -7 13 -460.507 556.352 0 7 -13 1909.86 657.008 0 -7 14 24646.2 2673.4 0 7 -14 24745.6 2279.04 0 -7 15 1055.51 683.694 0 7 -15 -259.142 445.801 0 7 -16 8514.35 1380.53 0 -7 16 9217.97 1740.91 0 8 0 49254.9 2667.47 0 8 0 50508.3 2053.75 0 8 1 20108.4 1211.18 0 8 -1 20535.6 1724.8 0 -8 -1 21653 1302.33 0 8 1 18972.5 1583.75 0 8 -2 2301.86 711.386 0 -8 -2 2415.15 476.91 0 8 2 2041.27 542.465 0 8 2 1304.85 290.28 0 8 -3 72671.6 2216.47 0 -8 -3 80834.3 2888.55 0 8 -3 80704 3651.55 0 8 3 77108 2385.86 0 8 3 75463 2966.3 0 8 -4 46515.6 2814.91 0 -8 -4 44095.7 2188.41 0 8 4 39488.9 1636.22 0 8 4 41208.8 2065.9 0 8 -4 38164.5 1605.71 0 8 5 82001.8 2739.78 0 8 5 78512.6 2375.77 0 -8 -5 81251.2 3211.66 0 8 -5 84171.6 3893.93 0 8 -6 1852.8 685.803 0 8 6 1137.93 286.568 0 -8 -6 2767.66 720.634 0 8 7 1698.41 362.746 0 8 -7 1747.65 585.876 0 8 -8 7515.79 1249.61 0 8 8 8273.06 813.827 0 8 -9 51015 3246.13 0 8 -10 3042.21 808.949 0 8 -11 9595.48 1461.32 0 8 -12 11903.7 1647.5 0 8 -13 28953.6 2545.09 0 -8 14 2121.11 899.108 0 8 -14 1234.94 511.463 0 -8 15 -1202.94 853.194 0 8 -15 618.442 519.423 0 -8 16 3445.64 1163.36 0 9 0 371.058 333.215 0 9 0 566.615 267.132 0 -9 -1 53305.3 2379.66 0 9 1 50631.5 2782.71 0 9 -1 49486.9 2894.42 0 9 1 55566.5 2172.45 0 9 -2 -179.939 406.167 0 -9 -2 274.193 163.305 0 9 2 536.12 315.7 0 9 2 313.691 169.074 0 9 -3 85879.6 4003.22 0 -9 -3 80761.1 3033 0 9 3 85465.9 2612.46 0 9 3 83082.9 3367.58 0 -9 -4 3402.35 647.177 0 9 4 2806.54 591.076 0 9 -4 3466.53 879.983 0 9 4 2713.19 432.096 0 9 5 20776.8 1193.18 0 9 5 20612.6 1467.33 0 9 -5 20052.4 1980.41 0 -9 -5 19562 1593.56 0 9 -6 1889.99 580.405 0 -9 -6 1363.66 422.432 0 -9 -7 56161 3016.45 0 9 -7 58394.1 3506.53 0 -9 -8 186.661 314.486 0 9 -8 -94.9036 362.556 0 -9 -9 6746.41 1137.34 0 9 -9 6897.92 1251.17 0 9 -10 4346.3 962.131 0 9 -11 42276 3164.95 0 9 -12 -139.174 355.237 0 9 -13 5423.38 1156.23 0 -9 14 -195.352 532.141 0 9 -14 -82.998 477.199 0 10 0 67706.8 2649.31 0 10 0 69411.9 3532.19 0 10 -1 22386.3 2025.66 0 10 1 23079.7 1439.9 0 10 1 22342.1 1932.83 0 10 2 1140.21 496.548 0 -10 -2 1350.38 424.342 0 10 2 576.006 217.608 0 10 -2 363.98 364.567 0 -10 -3 2479.37 563.853 0 10 -3 1891.06 752.526 0 10 3 2532.05 608.181 0 10 4 68662.4 3134.5 0 10 -4 65648.1 3699.94 0 -10 -4 68038.3 2999.44 0 10 5 2989.76 614.859 0 10 -5 2857.48 798.163 0 -10 -5 3007.6 718.788 0 -10 -6 2645.7 652.993 0 10 -6 2197.12 755.084 0 -10 -7 1032.07 532.179 0 10 -7 1065.74 546.77 0 10 -8 53026.7 3540 0 -10 -8 52328.1 3113.67 0 -10 -9 5523.91 1069.02 0 10 -9 4811.54 1062.94 0 -10 -10 4834.16 1022.49 0 10 -10 5658.97 1162.91 0 -10 -11 1241.6 536.949 0 10 -11 791.665 536.094 0 -10 -12 19687.3 2313.04 0 10 -12 22647.1 2403.7 0 -10 -13 2981.71 930.653 0 11 0 150.633 369.695 0 11 1 4140.88 878.468 0 11 -1 3810.23 861.023 0 11 -1 4197.96 743.955 0 11 -2 58908.4 3509.34 0 11 2 59429 3282.68 0 -11 -3 8428.39 1010.58 0 11 3 5774.58 993.071 0 11 -3 6950.77 1250.76 0 11 4 4632.67 859.187 0 11 -4 4234.09 995.76 0 -11 -4 3778.43 741.933 0 11 -5 1680.14 702.407 0 -11 -5 1533.33 521.34 0 11 -6 33934 2855.99 0 -11 -6 34025.8 2367.17 0 -11 -7 7564.18 1159.81 0 11 -7 6777.97 1333.72 0 11 -8 890.235 557.456 0 -11 -8 1489.02 587.172 0 -11 -9 4969.3 1045.55 0 11 -9 5121.38 1191.86 0 11 -10 14011.2 1990.53 0 -11 -10 15046.6 1914.58 0 -11 -11 2298.96 781.333 0 -11 -12 3401.8 945.722 0 12 0 470.534 388.723 0 12 -1 34486.6 2774.36 0 12 1 38903.8 2855.88 0 12 2 339.024 287.301 0 12 -2 575.652 525.076 0 12 3 11887.8 1525.25 0 12 -3 14715.4 1856.34 0 12 -4 595.825 396.095 0 12 -5 30764.5 2777.42 0 12 -6 -36.3688 391.766 0 12 -7 3760.27 1027.21 0 -12 -7 3561.57 818.13 0 -12 -8 2419.51 746.932 0 12 -8 2102.6 861.325 0 -12 -9 24442.1 2324.61 0 -12 -10 335.749 483.706 0 -12 -11 3971.02 1073.74 0 13 0 310.748 351.979 0 13 1 13708 1775.74 0 13 -1 11546.4 1673.36 0 13 2 24457.7 2342.18 0 13 -2 26486.6 2546.78 0 13 -3 11421.6 1727.05 0 13 -4 2004.17 745.994 0 13 -5 4349.01 1128.55 0 13 -6 8026.45 1463.83 0 14 0 33109.4 2932.54 0 14 -1 549.021 437.423 0 14 1 931.796 589.536 0 14 -2 -207.736 512.458 0 14 -3 -102.817 383.477 0 15 0 -20.5188 389.746 -1 0 18 24395 2754.98 -1 0 17 93.6859 406.851 -1 0 16 25460.7 2563.66 -1 0 15 -1067.77 623.098 -1 0 14 27433.9 2420.25 -1 0 13 7.35598 347.942 -1 0 12 73521.5 3638.9 1 0 -12 72122.9 2385.33 1 0 -11 200.982 162.299 -1 0 11 -246.293 392.448 -1 0 10 3464.25 706.687 1 0 -10 2080.39 364.824 1 0 -9 297.577 153.171 -1 0 9 90.2008 241.948 -1 0 8 125624 3820.19 1 0 -8 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