#------------------------------------------------------------------------------ #$Date: 2021-05-22 08:04:56 +0300 (Sat, 22 May 2021) $ #$Revision: 265452 $ #$URL: file:///home/coder/svn-repositories/cod/cif/2/24/38/2243837.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2243837 loop_ _publ_author_name 'Butcher, Ray J.' 'Purdy, Andrew P.' _publ_section_title ; \m-Methylene-bis[dibromido(diethyl ether-\kO)aluminium(III)]: crystal structure and chemical exchange in solution ; _journal_coeditor_code JQ2003 _journal_issue 6 _journal_name_full 'Acta Crystallographica Section E' _journal_page_first 647 _journal_page_last 652 _journal_paper_doi 10.1107/S2056989021005302 _journal_volume 77 _journal_year 2021 _chemical_formula_iupac '[Al2 Br4 (C H2) (C4 H10 O)2]' _chemical_formula_moiety 'C9 H22 Al2 Br4 O2' _chemical_formula_sum 'C9 H22 Al2 Br4 O2' _chemical_formula_weight 535.86 _chemical_name_systematic ; \m-Methylene-bis[dibromido(diethyl ether-\kO)aluminium(III)] ; _space_group_crystal_system monoclinic _space_group_IT_number 15 _space_group_name_Hall '-C 2yc' _space_group_name_H-M_alt 'C 1 2/c 1' _atom_sites_solution_hydrogens mixed _atom_sites_solution_primary direct _atom_sites_solution_secondary difmap _audit_creation_method SHELXL-2018/3 _cell_angle_alpha 90 _cell_angle_beta 95.646(3) _cell_angle_gamma 90 _cell_formula_units_Z 4 _cell_length_a 8.3872(6) _cell_length_b 12.1039(6) _cell_length_c 18.1504(12) _cell_measurement_reflns_used 4301 _cell_measurement_temperature 100(2) _cell_measurement_theta_max 32.46 _cell_measurement_theta_min 3.09 _cell_volume 1833.7(2) _computing_cell_refinement ; SAINT (Bruker, 2002) ; _computing_data_collection ; APEX2 (Bruker, 2005) ; _computing_data_reduction ; SAINT (Bruker, 2002) ; _computing_molecular_graphics ; SHELXTL (Sheldrick 2008) ; _computing_publication_material ; SHELXTL (Sheldrick 2008) ; _computing_structure_refinement ; SHELXL2018/3 (Sheldrick, 2015b) ; _computing_structure_solution ; SHELXT (Sheldrick 2015a) ; _diffrn_ambient_temperature 100(2) _diffrn_measured_fraction_theta_full 0.999 _diffrn_measured_fraction_theta_max 1.000 _diffrn_measurement_device_type 'Bruker APEXII CCD' _diffrn_measurement_method '\f and \w scans' _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_av_R_equivalents 0.0725 _diffrn_reflns_av_unetI/netI 0.0498 _diffrn_reflns_limit_h_max 10 _diffrn_reflns_limit_h_min -9 _diffrn_reflns_limit_k_max 15 _diffrn_reflns_limit_k_min -15 _diffrn_reflns_limit_l_max 23 _diffrn_reflns_limit_l_min -23 _diffrn_reflns_number 10600 _diffrn_reflns_theta_full 25.242 _diffrn_reflns_theta_max 27.099 _diffrn_reflns_theta_min 2.965 _exptl_absorpt_coefficient_mu 8.865 _exptl_absorpt_correction_T_max 0.7471 _exptl_absorpt_correction_T_min 0.2905 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details ; (SADABS; Sheldrick, 1996) ; _exptl_crystal_colour colorless _exptl_crystal_density_diffrn 1.941 _exptl_crystal_description plate _exptl_crystal_F_000 1032 _exptl_crystal_size_max 0.31 _exptl_crystal_size_mid 0.25 _exptl_crystal_size_min 0.08 _refine_diff_density_max 0.744 _refine_diff_density_min -0.726 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.073 _refine_ls_hydrogen_treatment mixed _refine_ls_matrix_type full _refine_ls_number_parameters 83 _refine_ls_number_reflns 2027 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.073 _refine_ls_R_factor_all 0.0396 _refine_ls_R_factor_gt 0.0305 _refine_ls_shift/su_max 0.001 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0337P)^2^+0.0465P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.0723 _refine_ls_wR_factor_ref 0.0759 _reflns_number_gt 1736 _reflns_number_total 2027 _reflns_threshold_expression 'I > 2\s(I)' _cod_data_source_file jq2003sup1.cif _cod_data_source_block I _cod_original_sg_symbol_H-M 'C 2/c' _cod_database_code 2243837 _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _shelx_hkl_file ; 1 -1 0 2.12 0.24 -2 2 0 258.16 19.18 2 -2 0 251.73 19.16 -3 3 0 150.62 11.13 3 -3 0 146.13 11.13 3 -3 0 144.52 11.10 -4 4 0 77.64 5.79 4 -4 0 73.59 5.84 4 -4 0 73.22 5.76 -5 5 0 117.22 8.51 5 -5 0 109.47 8.47 5 -5 0 104.22 8.55 -6 6 0 22.56 2.36 6 -6 0 24.26 2.38 6 -6 0 20.76 2.39 7 -7 0 15.73 1.76 7 -7 0 16.04 1.90 7 -7 0 8.23 2.29 8 -8 0 1.01 1.49 8 -8 0 2.13 1.83 8 -8 0 -1.85 2.79 8 -10 0 1.79 1.89 8 -10 0 -0.42 2.67 8 -10 0 -1.25 1.86 7 -9 0 3.95 1.62 7 -9 0 5.73 2.01 7 -9 0 4.08 2.11 -7 9 0 5.60 1.98 6 -8 0 10.21 1.52 6 -8 0 10.81 1.93 -6 8 0 12.20 1.76 5 -7 0 215.38 16.87 5 -7 0 217.55 16.77 -5 7 0 232.01 16.89 4 -6 0 4.91 0.74 4 -6 0 3.42 0.93 -4 6 0 4.97 1.08 3 -5 0 138.04 10.39 3 -5 0 137.08 10.44 -3 5 0 137.88 10.51 2 -4 0 902.30 68.50 2 -4 0 907.73 68.47 -2 4 0 926.34 68.55 1 -3 0 37.22 2.83 1 -3 0 37.58 2.87 -1 3 0 37.64 2.98 0 -2 0 516.29 38.85 0 -2 0 465.18 38.86 0 2 0 529.99 38.89 0 2 0 558.38 38.85 1 1 0 2.69 0.32 1 1 0 2.55 0.28 1 1 0 2.43 0.28 2 0 0 3.07 0.40 2 0 0 4.19 0.76 3 -1 0 43.19 3.24 3 -1 0 39.53 3.38 4 -2 0 106.20 8.20 4 -2 0 109.41 8.31 4 -2 0 108.13 8.14 5 -3 0 0.28 1.11 5 -3 0 1.59 0.54 5 -3 0 2.71 0.78 6 -4 0 145.35 10.95 6 -4 0 140.85 11.21 6 -4 0 145.69 11.02 7 -5 0 2.70 1.31 7 -5 0 2.42 1.07 7 -5 0 4.18 1.88 8 -6 0 -3.42 2.28 8 -6 0 -3.84 1.49 8 -6 0 0.71 1.68 9 -7 0 6.81 3.11 9 -7 0 14.10 2.33 7 -11 0 16.80 2.92 -7 11 0 19.63 2.69 6 -10 0 14.99 2.00 6 -10 0 20.05 2.49 -6 10 0 22.87 2.52 5 -9 0 92.57 8.14 5 -9 0 112.97 8.11 4 -8 0 148.94 11.29 4 -8 0 143.59 11.16 -4 8 0 150.26 11.40 3 -7 0 72.11 5.45 3 -7 0 67.99 5.30 -3 7 0 69.68 5.61 2 -6 0 306.47 22.93 2 -6 0 306.56 22.87 -2 6 0 300.10 23.02 1 -5 0 17.16 1.39 1 -5 0 18.54 1.51 -1 5 0 18.72 1.81 0 -4 0 27.40 2.20 0 4 0 27.69 2.39 0 4 0 29.64 2.21 1 3 0 35.29 2.78 1 3 0 36.83 2.75 1 3 0 35.57 2.90 2 2 0 232.44 17.73 2 2 0 234.67 17.71 2 2 0 238.65 17.71 3 1 0 38.29 2.91 3 1 0 36.71 3.34 4 0 0 332.16 28.57 4 0 0 419.71 28.43 5 -1 0 12.54 1.26 5 -1 0 8.91 1.88 6 -2 0 12.41 1.47 6 -2 0 14.82 2.11 7 -3 0 29.93 3.29 8 -4 0 1.46 1.56 8 -4 0 6.12 2.55 9 -5 0 1.42 1.92 9 -5 0 4.54 2.95 6 -12 0 8.26 2.33 -6 12 0 7.10 2.26 5 -11 0 9.91 1.93 -5 11 0 11.43 2.16 4 -10 0 123.03 9.43 -4 10 0 119.61 9.63 3 -9 0 71.49 5.75 -3 9 0 75.03 6.50 2 -8 0 10.48 0.88 2 -8 0 8.99 1.12 -2 8 0 8.35 1.55 1 -7 0 94.66 7.37 1 -7 0 100.60 7.46 -1 7 0 98.77 7.69 0 -6 0 14.63 1.74 0 -6 0 15.97 1.41 0 6 0 17.67 1.96 1 5 0 16.04 1.43 1 5 0 18.79 1.53 1 5 0 15.87 1.79 2 4 0 849.25 63.75 2 4 0 844.38 63.81 2 4 0 852.48 63.74 3 3 0 135.21 10.33 3 3 0 136.71 10.31 4 2 0 103.12 7.82 4 2 0 103.63 7.99 4 2 0 100.89 7.77 5 1 0 13.02 1.31 5 1 0 8.79 2.23 6 0 0 63.60 4.87 6 0 0 53.29 5.78 7 -1 0 3.22 2.65 7 -1 0 5.63 1.32 8 -2 0 5.32 2.89 8 -2 0 5.74 1.61 9 -3 0 45.65 4.11 9 -3 0 31.16 4.73 10 -4 0 2.84 3.66 10 -4 0 1.94 2.20 5 -13 0 0.35 2.01 -5 13 0 2.51 2.27 4 -12 0 6.87 1.77 -4 12 0 7.87 2.12 3 -11 0 137.67 10.58 -3 11 0 135.58 10.79 2 -10 0 80.42 6.12 -2 10 0 75.21 6.46 1 -9 0 98.94 7.57 1 -9 0 92.89 7.42 -1 9 0 107.68 8.20 0 -8 0 204.86 16.52 0 -8 0 221.57 16.50 0 8 0 229.41 16.70 -1 -7 0 91.34 7.32 -1 -7 0 88.91 7.57 1 7 0 102.37 7.37 1 7 0 99.16 7.32 1 7 0 96.70 7.58 2 6 0 271.22 21.06 2 6 0 280.06 20.92 2 6 0 282.14 20.96 3 5 0 128.13 9.75 3 5 0 126.60 9.60 3 5 0 124.97 9.64 4 4 0 69.16 5.27 4 4 0 67.16 5.33 4 4 0 66.22 5.29 5 3 0 0.85 1.25 5 3 0 2.58 0.72 5 3 0 3.20 0.90 6 2 0 9.22 1.27 6 2 0 12.24 2.23 7 1 0 6.49 1.34 7 1 0 5.74 2.96 8 0 0 97.82 9.17 8 0 0 97.74 7.80 9 -1 0 21.72 2.55 9 -1 0 24.54 4.30 10 -2 0 -0.95 2.13 10 -2 0 0.52 4.24 4 -14 0 36.54 3.76 -4 14 0 39.22 4.82 3 -13 0 69.15 5.72 -3 13 0 65.23 6.25 2 -12 0 3.89 1.40 -2 12 0 4.55 2.01 1 -11 0 34.24 3.19 -1 11 0 36.28 3.78 0 -10 0 83.48 7.25 0 -10 0 99.78 7.34 0 10 0 103.34 7.68 -1 -9 0 79.49 7.29 -1 -9 0 91.39 6.92 1 9 0 94.42 6.90 -2 -8 0 13.72 1.84 2 8 0 6.66 1.58 2 8 0 8.80 1.24 2 8 0 7.78 0.99 3 7 0 65.42 5.07 3 7 0 62.05 4.96 3 7 0 64.30 5.26 4 6 0 3.92 1.02 4 6 0 3.18 1.24 4 6 0 4.23 0.86 5 5 0 105.69 8.06 5 5 0 105.15 8.02 5 5 0 100.33 8.01 6 4 0 132.86 10.33 6 4 0 141.85 10.53 6 4 0 133.24 10.40 7 3 0 29.74 3.51 7 3 0 33.52 3.04 8 2 0 2.44 2.95 8 2 0 9.74 1.66 9 1 0 12.75 4.07 9 1 0 22.12 2.48 10 0 0 3.64 4.33 10 0 0 2.56 2.15 2 -14 0 18.11 2.36 -2 14 0 16.87 2.95 1 -13 0 39.49 3.78 -1 13 0 39.02 4.41 0 -12 0 66.44 5.42 0 -12 0 70.12 5.69 0 12 0 77.47 6.33 -1 -11 0 30.70 3.10 -1 -11 0 31.62 2.95 1 11 0 32.21 3.70 -2 -10 0 70.94 5.82 -2 -10 0 59.22 6.57 2 10 0 77.10 6.26 2 10 0 80.12 5.78 3 9 0 66.44 5.27 3 9 0 61.88 5.57 4 8 0 129.30 10.18 4 8 0 132.88 10.29 4 8 0 138.88 10.48 5 7 0 205.31 15.46 5 7 0 200.98 15.53 5 7 0 201.90 15.39 6 6 0 21.02 2.33 6 6 0 22.70 2.41 6 6 0 18.26 2.40 7 5 0 3.45 1.09 7 5 0 3.64 1.70 7 5 0 2.83 1.39 8 4 0 2.33 1.52 8 4 0 0.30 2.27 9 3 0 29.86 4.34 9 3 0 37.16 3.75 10 2 0 -1.89 2.01 10 2 0 -0.41 3.81 1 -15 0 25.59 2.92 -1 15 0 26.60 3.61 0 -14 0 165.23 12.70 0 14 0 162.49 13.10 -1 -13 0 34.08 3.48 -1 -13 0 40.62 3.60 1 13 0 38.13 4.36 -2 -12 0 3.96 1.38 -2 -12 0 -0.22 2.45 2 12 0 6.45 2.15 -3 -11 0 106.51 10.15 3 11 0 127.40 9.39 3 11 0 124.76 9.82 4 10 0 107.61 8.61 4 10 0 110.27 9.04 4 10 0 118.32 9.05 5 9 0 97.99 8.07 5 9 0 97.04 7.71 5 9 0 102.55 7.87 6 8 0 10.87 1.79 6 8 0 11.44 1.54 6 8 0 10.30 1.91 7 7 0 12.03 1.80 7 7 0 12.24 1.89 7 7 0 13.33 1.83 8 6 0 0.07 1.91 8 6 0 -0.26 1.58 8 6 0 0.98 1.24 9 5 0 5.76 2.51 9 5 0 5.34 2.64 10 4 0 3.50 2.03 -1 -15 0 27.57 2.96 1 15 0 26.24 3.61 -2 -14 0 11.85 2.02 -2 -14 0 13.26 2.45 2 14 0 15.02 2.90 -3 -13 0 52.70 6.38 -3 -13 0 55.87 5.11 3 13 0 58.80 4.90 3 13 0 64.89 5.92 -4 -12 0 7.10 3.35 4 12 0 7.70 1.45 4 12 0 7.56 2.03 4 12 0 5.63 2.42 5 11 0 11.26 1.60 5 11 0 10.75 2.41 5 11 0 11.01 2.13 6 10 0 21.90 2.52 6 10 0 16.94 2.03 6 10 0 19.28 2.67 7 9 0 3.32 1.47 7 9 0 4.21 1.88 7 9 0 2.30 1.84 8 8 0 2.08 1.70 8 8 0 5.32 1.83 8 8 0 1.49 1.92 9 7 0 9.52 2.24 9 7 0 11.68 2.38 -4 -14 0 29.66 4.67 -4 -14 0 23.34 3.03 4 14 0 41.12 4.88 4 14 0 34.34 3.23 -5 -13 0 0.58 3.91 5 13 0 1.74 3.35 5 13 0 0.31 1.57 5 13 0 -1.73 2.25 -6 -12 0 2.78 3.79 6 12 0 4.89 2.32 6 12 0 4.99 1.55 6 12 0 5.18 2.51 7 11 0 16.08 2.80 7 11 0 16.32 3.01 7 11 0 16.86 2.10 8 10 0 -0.38 2.02 8 10 0 3.08 2.24 8 10 -1 9.01 1.76 8 10 -1 10.55 2.22 8 10 -1 5.89 2.23 7 11 -1 0.82 2.17 7 11 -1 2.97 2.17 7 11 -1 2.58 1.46 6 12 -1 66.92 6.07 6 12 -1 61.66 5.81 6 12 -1 59.92 5.30 5 13 -1 8.13 1.62 5 13 -1 5.93 3.52 5 13 -1 13.13 2.52 -5 -13 1 6.84 3.93 4 14 -1 6.65 2.70 4 14 -1 1.64 2.59 -4 -14 1 -0.18 1.91 -4 -14 1 -1.35 3.75 9 7 -1 8.94 2.11 9 7 -1 7.97 2.07 8 8 -1 81.03 6.73 8 8 -1 76.95 6.75 8 8 -1 85.83 6.72 7 9 -1 9.33 1.51 7 9 -1 5.16 1.88 7 9 -1 7.57 1.83 6 10 -1 36.03 3.73 6 10 -1 32.72 4.08 6 10 -1 36.82 3.31 5 11 -1 3.09 1.79 5 11 -1 2.36 2.11 5 11 -1 1.02 1.21 4 12 -1 37.87 3.73 4 12 -1 33.49 3.10 4 12 -1 36.63 4.26 -4 -12 1 25.84 2.96 -4 -12 1 35.24 4.38 3 13 -1 1.69 2.24 -3 -13 1 -3.69 3.18 -3 -13 1 -0.30 1.50 2 14 -1 1.29 2.36 -2 -14 1 -2.17 1.95 -2 -14 1 1.14 1.62 1 15 -1 8.60 2.76 -1 -15 1 7.05 2.00 10 4 -1 21.16 3.57 10 4 -1 19.93 2.61 9 5 -1 0.00 2.27 8 6 -1 80.98 6.71 8 6 -1 77.20 6.38 8 6 -1 72.44 6.53 -8 -6 1 86.75 6.42 7 7 -1 18.00 1.92 7 7 -1 16.17 1.99 7 7 -1 13.56 1.93 6 8 -1 27.36 2.61 6 8 -1 25.71 2.55 6 8 -1 23.03 3.02 5 9 -1 9.29 1.98 5 9 -1 10.85 1.72 5 9 -1 11.95 1.40 4 10 -1 2.46 1.83 4 10 -1 4.17 1.49 4 10 -1 2.36 1.03 3 11 -1 2.45 1.87 3 11 -1 3.28 1.08 3 11 -1 4.94 1.53 -3 -11 1 3.95 2.68 -3 -11 1 1.65 1.21 2 12 -1 79.82 6.70 -2 -12 1 60.83 6.91 -2 -12 1 79.34 6.13 1 13 -1 37.50 4.08 -1 -13 1 28.91 3.04 -1 -13 1 34.94 3.34 0 14 -1 18.95 2.95 0 -14 1 16.28 2.24 -1 15 -1 6.25 2.72 1 -15 1 3.78 1.97 10 2 -1 16.73 4.14 10 2 -1 21.77 2.66 9 3 -1 4.35 1.69 9 3 -1 1.04 2.91 8 4 -1 5.89 2.20 8 4 -1 5.91 1.58 7 5 -1 136.18 10.40 7 5 -1 130.85 10.21 7 5 -1 133.76 10.32 6 6 -1 16.24 2.12 6 6 -1 13.80 1.76 6 6 -1 17.79 1.88 5 7 -1 7.01 1.49 5 7 -1 6.08 1.07 4 8 -1 30.52 2.87 4 8 -1 29.53 3.21 4 8 -1 30.79 2.65 3 9 -1 2.52 1.15 3 9 -1 1.81 0.84 3 9 -1 -1.47 1.48 2 10 -1 18.92 2.02 2 10 -1 21.31 2.47 -2 -10 1 19.55 2.14 -2 -10 1 20.50 2.79 1 11 -1 5.10 1.90 -1 -11 1 4.82 1.74 -1 -11 1 7.72 1.25 0 12 -1 115.83 9.34 0 -12 1 115.07 8.99 -1 13 -1 0.72 2.01 1 -13 1 0.68 1.44 -2 14 -1 15.34 2.85 2 -14 1 15.92 2.45 10 0 -1 2.14 2.01 10 0 -1 3.67 4.22 9 1 -1 44.10 5.76 9 1 -1 58.25 4.79 8 2 -1 6.12 1.49 8 2 -1 -0.42 2.81 7 3 -1 66.51 6.41 7 3 -1 65.23 5.29 6 4 -1 15.34 1.82 6 4 -1 20.83 2.01 6 4 -1 18.74 1.98 5 5 -1 1.85 0.96 5 5 -1 -0.05 0.95 5 5 -1 2.24 0.91 4 6 -1 29.96 2.68 4 6 -1 29.38 2.84 4 6 -1 31.12 2.55 3 7 -1 2.58 0.66 3 7 -1 2.14 1.23 3 7 -1 1.09 0.88 2 8 -1 62.56 4.95 2 8 -1 62.03 5.26 2 8 -1 65.71 5.02 -1 -9 1 2.06 0.82 -1 -9 1 1.78 1.92 0 10 -1 27.36 3.20 0 -10 1 27.01 2.45 0 -10 1 35.54 2.69 -1 11 -1 5.99 1.78 1 -11 1 5.18 1.24 -2 12 -1 -0.04 1.89 2 -12 1 1.81 1.37 -3 13 -1 16.12 2.55 3 -13 1 11.16 2.09 -4 14 -1 23.13 3.27 4 -14 1 27.47 3.04 10 -2 -1 14.92 2.80 9 -1 -1 64.77 5.58 9 -1 -1 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8.55 -6 -4 4 115.36 8.82 5 5 -4 2.35 0.99 5 5 -4 3.07 0.75 5 5 -4 4.93 0.88 -5 -5 4 5.13 1.19 4 6 -4 8.35 1.31 4 6 -4 10.08 1.08 4 6 -4 8.84 0.95 3 7 -4 16.78 1.45 3 7 -4 13.45 1.58 3 7 -4 14.98 1.75 2 8 -4 7.82 0.95 2 8 -4 7.98 1.45 2 8 -4 7.38 0.90 -2 -8 4 6.90 0.97 1 9 -4 47.58 4.34 1 9 -4 53.16 3.95 -1 -9 4 47.55 3.99 0 10 -4 40.60 3.94 -1 11 -4 158.99 13.10 1 -11 4 178.55 12.92 -2 12 -4 7.86 2.08 2 -12 4 9.03 1.71 -3 13 -4 1.31 2.11 3 -13 4 0.56 1.90 -4 14 -4 0.95 2.40 4 -14 4 2.99 2.30 10 -2 -4 53.02 4.95 10 -2 -4 44.94 5.96 9 -1 -4 7.44 3.71 9 -1 -4 4.06 1.53 8 0 -4 183.89 15.99 8 0 -4 207.40 15.16 7 1 -4 4.17 2.54 7 1 -4 3.46 1.04 6 2 -4 2.65 1.57 6 2 -4 1.42 0.94 5 3 -4 31.38 2.63 5 3 -4 29.06 2.50 -5 -3 4 29.97 2.78 4 4 -4 4.60 0.77 4 4 -4 3.58 0.69 4 4 -4 4.07 0.87 -4 -4 4 5.35 1.01 3 5 -4 1.20 0.55 3 5 -4 2.08 0.48 3 5 -4 2.09 0.83 2 6 -4 46.67 3.56 2 6 -4 45.65 3.80 2 6 -4 48.05 3.62 -2 -6 4 43.55 3.57 1 7 -4 177.55 13.26 1 7 -4 176.13 13.08 -1 -7 4 166.78 13.10 0 8 -4 0.58 1.09 0 -8 4 0.20 0.69 -1 9 -4 1.77 1.24 1 -9 4 1.13 0.88 -2 10 -4 2.04 1.50 2 -10 4 1.92 1.16 -3 11 -4 4.55 1.74 3 -11 4 3.02 1.54 -4 12 -4 2.84 2.05 4 -12 4 2.70 1.86 5 -13 4 84.31 7.54 10 -4 -4 74.92 8.05 9 -3 -4 -5.50 3.32 9 -3 -4 1.24 1.53 8 -2 -4 40.81 4.72 8 -2 -4 45.04 3.87 7 -1 -4 2.13 2.61 7 -1 -4 3.22 1.01 6 0 -4 2.02 2.23 6 0 -4 1.17 0.76 5 1 -4 14.30 2.02 5 1 -4 15.10 1.30 -5 -1 4 9.26 1.33 4 2 -4 101.21 8.14 4 2 -4 118.37 8.21 -4 -2 4 103.12 8.30 3 3 -4 126.76 10.24 3 3 -4 133.34 10.30 3 3 -4 138.47 10.22 -3 -3 4 144.01 10.33 2 4 -4 103.28 7.73 2 4 -4 102.42 7.61 2 4 -4 97.02 7.62 1 5 -4 8.95 1.06 1 5 -4 7.72 0.79 -1 -5 4 7.51 0.82 0 6 -4 91.98 7.03 0 -6 4 88.73 6.86 -1 7 -4 144.79 11.34 1 -7 4 150.83 11.21 -2 8 -4 13.13 1.65 2 -8 4 11.82 1.36 -3 9 -4 69.38 5.89 3 -9 4 73.98 5.71 -4 10 -4 4.17 1.69 4 -10 4 5.30 1.58 -5 11 -4 271.71 21.61 5 -11 4 296.26 21.78 5 -11 4 278.21 21.57 -6 12 -4 2.46 2.29 6 -12 4 1.82 2.69 6 -12 4 2.08 2.50 9 -5 -4 12.69 3.39 9 -5 -4 15.55 2.06 8 -4 -4 9.22 2.68 8 -4 -4 8.63 1.55 7 -3 -4 31.74 3.50 7 -3 -4 34.88 3.06 6 -2 -4 1.20 1.70 6 -2 -4 2.00 0.85 5 -1 -4 13.19 1.47 5 -1 -4 18.27 2.00 4 0 -4 357.28 25.16 4 0 -4 324.68 25.29 -4 0 4 320.16 25.18 3 1 -4 102.95 8.04 3 1 -4 110.46 8.16 2 2 -4 39.60 3.00 2 2 -4 37.45 3.03 -2 -2 4 42.13 3.18 1 3 -4 11.00 0.99 1 3 -4 14.07 1.28 -1 -3 4 12.91 1.28 -1 -3 4 12.43 0.98 0 4 -4 91.86 7.29 0 4 -4 102.32 7.42 0 -4 4 97.12 7.32 -1 5 -4 29.07 2.46 1 -5 4 27.58 2.28 -2 6 -4 19.28 1.94 2 -6 4 15.68 1.62 -3 7 -4 263.12 19.77 3 -7 4 257.86 19.70 -4 8 -4 23.51 2.78 4 -8 4 24.11 2.66 4 -8 4 26.08 3.00 -5 9 -4 66.76 5.63 5 -9 4 65.06 5.79 5 -9 4 64.42 5.63 6 -10 4 0.28 2.12 6 -10 4 0.24 2.11 7 -11 4 2.46 2.51 7 -11 4 2.08 2.74 9 -7 -4 41.12 3.93 9 -7 -4 37.98 4.51 8 -6 -4 0.22 1.35 8 -6 -4 1.49 2.30 -8 6 4 -2.10 0.92 7 -5 -4 50.48 4.73 7 -5 -4 48.20 4.15 -7 5 4 50.32 4.08 6 -4 -4 127.03 9.74 6 -4 -4 123.51 9.94 -6 4 4 130.75 9.76 5 -3 -4 32.32 2.70 5 -3 -4 33.88 2.97 -5 3 4 32.33 2.86 4 -2 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78.95 5.95 1 -1 -4 80.57 5.98 -1 1 4 77.15 6.13 0 0 -4 70.41 5.65 0 0 4 78.23 5.62 -1 1 -4 361.56 26.65 1 -1 4 346.61 26.66 -2 2 -4 366.25 29.06 2 -2 4 394.13 29.12 2 -2 4 398.29 29.07 3 -3 4 122.68 9.51 3 -3 4 126.26 9.52 4 -4 4 77.88 5.99 4 -4 4 74.33 6.02 5 -5 4 39.73 3.16 5 -5 4 32.41 3.25 5 -5 4 25.35 3.32 6 -6 4 39.72 4.37 6 -6 4 48.57 4.13 6 -6 4 44.10 4.22 7 -7 4 242.79 17.06 7 -7 4 198.73 17.00 7 -7 4 219.25 17.11 8 -8 4 3.88 2.46 8 -8 4 3.89 2.70 8 -8 4 5.23 2.51 8 -10 -4 59.47 5.94 8 -10 -4 55.23 4.98 -8 10 4 56.18 5.21 7 -9 -4 65.27 5.30 7 -9 -4 62.60 5.86 6 -8 -4 0.17 1.47 6 -8 -4 1.01 0.99 -6 8 4 0.80 1.57 5 -7 -4 5.40 0.92 5 -7 -4 5.52 1.21 -5 7 4 5.38 1.62 4 -6 -4 7.62 1.13 4 -6 -4 9.01 0.96 -4 6 4 10.57 1.67 3 -5 -4 1.57 0.50 3 -5 -4 1.66 0.63 -3 5 4 1.73 1.25 2 -4 -4 105.55 7.91 2 -4 -4 104.17 7.91 -2 4 4 103.69 8.25 1 -3 -4 12.57 1.13 1 -3 -4 13.46 1.20 -1 3 4 13.78 1.14 -1 3 4 14.38 1.50 0 -2 -4 25.59 2.29 0 2 4 29.66 2.39 0 2 4 28.48 2.17 -1 -1 -4 332.10 26.83 1 1 4 369.32 26.78 1 1 4 366.58 26.89 2 0 4 142.13 10.26 2 0 4 126.71 10.52 3 -1 4 78.90 7.02 3 -1 4 104.77 7.12 4 -2 4 125.60 10.22 4 -2 4 139.83 10.24 5 -3 4 310.51 22.29 5 -3 4 277.02 22.26 6 -4 4 65.32 5.76 7 -5 4 83.99 6.96 7 -5 4 80.24 6.93 8 -6 4 3.46 2.51 8 -6 4 6.14 2.39 8 -6 4 0.97 2.50 9 -7 4 -1.93 3.02 9 -7 4 -3.47 2.69 7 -11 -4 16.85 2.77 -7 11 4 17.88 2.70 6 -10 -4 14.81 2.20 6 -10 -4 16.36 1.71 -6 10 4 15.70 2.45 5 -9 -4 17.21 1.83 5 -9 -4 17.57 1.99 -5 9 4 16.58 2.42 4 -8 -4 31.41 2.76 4 -8 -4 30.85 2.54 -4 8 4 28.31 3.47 3 -7 -4 15.60 1.64 3 -7 -4 14.25 1.40 -3 7 4 16.55 2.11 2 -6 -4 46.07 3.65 2 -6 -4 47.31 3.71 -2 6 4 48.97 4.28 1 -5 -4 12.40 1.17 1 -5 -4 9.06 1.04 -1 5 4 8.46 1.52 0 -4 -4 96.46 7.69 0 4 4 102.93 7.60 0 4 4 101.29 7.78 -1 -3 -4 248.15 21.11 1 3 4 290.00 21.02 1 3 4 298.33 21.11 -2 -2 -4 372.61 28.58 2 2 4 384.69 28.55 3 1 4 93.58 7.74 3 1 4 104.17 7.86 3 1 4 103.66 7.76 4 0 4 78.46 6.18 4 0 4 76.77 6.45 4 0 4 78.33 6.30 5 -1 4 86.16 7.75 5 -1 4 97.16 7.53 5 -1 4 103.88 7.80 6 -2 4 20.80 2.27 6 -2 4 15.90 2.45 6 -2 4 16.49 2.66 7 -3 4 3.52 2.33 7 -3 4 2.02 2.15 7 -3 4 4.91 1.97 8 -4 4 10.68 2.43 8 -4 4 9.21 2.67 9 -5 4 -3.43 2.54 9 -5 4 -0.95 3.02 6 -12 -4 4.40 2.01 6 -12 -4 0.07 1.21 -6 12 4 0.11 2.28 5 -11 -4 45.02 4.35 5 -11 -4 45.46 3.79 -5 11 4 48.21 5.00 4 -10 -4 73.87 5.80 4 -10 -4 76.41 6.03 -4 10 4 75.24 6.65 3 -9 -4 2.53 0.97 3 -9 -4 1.64 0.64 -3 9 4 -0.37 1.76 2 -8 -4 7.92 0.88 2 -8 -4 7.14 1.01 -2 8 4 7.31 1.95 1 -7 -4 177.27 13.56 1 -7 -4 179.07 13.57 -1 7 4 181.85 13.90 0 -6 -4 89.38 7.03 0 6 4 92.51 6.87 0 6 4 87.49 7.22 -1 -5 -4 22.79 2.71 1 5 4 25.90 2.77 1 5 4 28.08 2.18 -2 -4 -4 101.34 8.37 2 4 4 116.76 8.17 2 4 4 110.27 8.33 2 4 4 99.16 8.25 3 3 4 119.51 8.77 3 3 4 114.79 8.62 3 3 4 102.70 8.66 4 2 4 135.78 10.63 4 2 4 131.58 10.73 4 2 4 145.28 10.57 5 1 4 110.92 8.15 5 1 4 100.65 8.62 5 1 4 102.78 8.30 6 0 4 4.47 2.63 6 0 4 6.13 1.64 6 0 4 5.60 1.03 7 -1 4 32.09 3.81 7 -1 4 33.96 3.57 8 -2 4 44.83 4.77 8 -2 4 46.22 4.67 9 -3 4 25.42 5.52 9 -3 4 30.11 3.49 5 -13 -4 25.40 3.05 -5 13 4 29.13 3.63 4 -12 -4 3.30 1.61 4 -12 -4 2.10 0.86 -4 12 4 2.51 2.42 3 -11 -4 38.84 3.23 3 -11 -4 43.40 3.66 -3 11 4 38.96 4.71 2 -10 -4 66.05 5.34 2 -10 -4 66.43 5.17 -2 10 4 68.66 6.11 1 -9 -4 49.78 4.04 1 -9 -4 49.29 4.03 -1 9 4 52.37 4.82 0 -8 -4 -1.34 1.19 0 -8 -4 -0.10 0.72 0 8 4 -0.21 1.67 0 8 4 0.95 0.70 -1 -7 -4 126.24 10.41 1 7 4 137.65 10.14 1 7 4 135.24 10.51 -2 -6 -4 14.50 2.00 2 6 4 15.09 2.07 2 6 4 16.06 1.53 -3 -5 -4 96.58 7.29 3 5 4 83.74 7.23 3 5 4 90.74 7.08 3 5 4 90.80 6.95 4 4 4 66.39 5.52 4 4 4 71.90 5.41 4 4 4 63.83 5.55 5 3 4 281.43 22.37 5 3 4 289.90 22.45 5 3 4 309.83 22.32 6 2 4 22.66 2.45 6 2 4 19.47 2.44 6 2 4 23.43 3.04 7 1 4 33.34 4.21 7 1 4 38.12 3.77 8 0 4 115.44 10.12 8 0 4 117.70 9.39 9 -1 4 29.47 4.34 9 -1 4 29.72 3.41 10 -2 4 25.79 4.39 10 -2 4 24.13 3.86 4 -14 -4 43.05 4.62 -4 14 4 50.35 5.67 3 -13 -4 2.31 2.86 3 -13 -4 3.79 0.82 -3 13 4 1.06 2.56 2 -12 -4 6.59 1.49 2 -12 -4 7.29 0.95 -2 12 4 8.54 2.61 1 -11 -4 34.43 3.32 1 -11 -4 36.55 3.14 -1 11 4 42.13 4.65 0 -10 -4 40.98 3.41 0 -10 -4 35.76 3.65 0 10 4 41.38 4.59 -1 -9 -4 0.56 1.76 1 9 4 -0.14 1.95 1 9 4 -0.01 0.85 -2 -8 -4 6.04 2.11 2 8 4 8.41 2.06 2 8 4 10.97 1.18 -3 -7 -4 215.39 17.23 3 7 4 220.65 17.26 3 7 4 234.07 17.06 3 7 4 224.81 16.96 4 6 4 26.40 3.28 4 6 4 28.06 2.95 4 6 4 29.32 2.64 5 5 4 36.44 3.47 5 5 4 33.28 3.60 6 4 4 102.86 7.88 6 4 4 90.71 8.13 6 4 4 98.80 7.86 7 3 4 10.08 1.92 7 3 4 1.76 2.74 7 3 4 6.09 1.45 8 2 4 35.67 4.89 8 2 4 50.83 4.63 9 1 4 33.05 4.42 9 1 4 28.22 3.41 10 0 4 2.88 2.58 10 0 4 5.78 3.84 2 -14 -4 9.70 1.95 -2 14 4 9.98 3.09 1 -13 -4 2.34 0.92 1 -13 -4 2.11 1.45 -1 13 4 -0.02 2.62 0 -12 -4 4.75 1.36 0 -12 -4 4.13 1.40 0 12 4 6.78 2.57 -1 -11 -4 154.79 11.99 -1 -11 -4 159.83 12.28 1 11 4 153.11 11.94 1 11 4 159.29 13.10 -2 -10 -4 -0.23 2.21 2 10 4 1.98 1.04 2 10 4 0.88 2.14 -3 -9 -4 55.09 5.80 3 9 4 59.95 5.79 3 9 4 63.71 4.91 -4 -8 -4 20.61 2.99 4 8 4 21.22 2.37 4 8 4 17.99 3.25 4 8 4 26.21 2.50 5 7 4 1.33 1.67 5 7 4 0.81 1.97 5 7 4 1.46 1.34 6 6 4 42.13 4.44 6 6 4 48.12 4.51 6 6 4 43.93 4.29 7 5 4 91.92 7.47 7 5 4 90.42 7.29 7 5 4 84.17 7.68 8 4 4 11.32 2.31 8 4 4 7.55 3.12 9 3 4 24.04 4.35 9 3 4 29.55 3.88 10 2 4 23.63 3.39 10 2 4 24.64 4.71 1 -15 -4 11.50 2.12 -1 15 4 8.37 3.22 0 -14 -4 1.31 1.61 0 -14 -4 3.49 1.30 0 14 4 1.22 2.78 -1 -13 -4 39.76 4.30 -1 -13 -4 43.74 3.96 1 13 4 41.48 5.18 -2 -12 -4 8.37 2.60 -2 -12 -4 6.27 1.51 2 12 4 7.46 1.43 2 12 4 6.57 2.71 -3 -11 -4 10.20 2.92 3 11 4 3.35 2.46 3 11 4 2.68 1.28 -4 -10 -4 5.14 2.80 4 10 4 2.16 2.42 4 10 4 3.87 1.30 -5 -9 -4 56.09 6.07 5 9 4 55.41 5.64 5 9 4 57.63 5.36 5 9 4 60.30 4.91 6 8 4 3.38 2.23 6 8 4 3.83 1.92 6 8 4 2.11 1.71 7 7 4 227.96 17.43 7 7 4 220.44 17.41 7 7 4 228.52 17.36 8 6 4 9.54 2.23 8 6 4 5.13 2.86 8 6 4 5.53 1.83 9 5 4 3.55 2.42 9 5 4 0.34 4.46 -1 -15 -4 3.81 1.74 -1 -15 -4 4.18 1.85 1 15 4 2.73 3.14 -2 -14 -4 34.57 3.79 -2 -14 -4 39.95 3.98 2 14 4 34.32 4.38 -3 -13 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1.86 -3 -1 20 -4.66 6.99 2 2 -20 58.37 5.26 -2 -2 20 57.26 8.26 1 3 -20 41.08 4.04 -1 -3 20 36.28 6.58 0 4 -20 75.29 6.27 -1 5 -20 0.76 1.68 1 -5 20 3.39 1.29 1 -5 20 0.47 4.88 -2 6 -20 -0.62 1.58 2 -6 20 0.57 5.05 2 -6 20 1.69 1.67 5 -3 -20 59.17 5.19 -5 3 20 40.45 6.92 4 -2 -20 29.18 3.24 -4 2 20 29.77 7.22 3 -1 -20 -1.25 1.87 -3 1 20 2.64 6.97 2 0 -20 74.33 6.48 -2 0 20 79.15 10.14 1 1 -20 7.61 1.94 -1 -1 20 12.00 6.78 0 2 -20 67.69 5.52 0 -2 20 55.71 8.20 0 -2 20 62.38 5.05 -1 3 -20 -3.95 1.65 1 -3 20 0.03 1.24 -2 4 -20 -2.23 1.63 2 -4 20 7.72 5.24 2 -4 20 -0.86 1.47 -3 5 -20 10.63 1.93 3 -5 20 11.26 5.65 3 -5 20 12.43 2.15 5 -5 -20 12.79 2.54 -5 5 20 14.92 4.96 4 -4 -20 9.14 2.35 4 -4 -20 8.46 1.49 3 -3 -20 3.05 1.07 3 -3 -20 -0.33 2.18 -3 3 20 3.72 6.32 2 -2 -20 60.56 5.57 2 -2 -20 64.67 4.95 -2 2 20 52.06 9.11 1 -1 -20 8.62 2.05 -1 1 20 6.05 1.11 -1 1 20 5.40 7.35 0 0 -20 49.68 4.56 0 0 20 48.16 4.12 0 0 20 48.62 8.76 -1 1 -20 -3.59 1.73 1 -1 20 -0.50 1.31 1 -1 20 -1.47 6.49 -2 2 -20 16.53 2.34 2 -2 20 21.47 10.64 2 -2 20 18.30 2.14 -3 3 -20 34.08 3.62 3 -3 20 25.88 6.55 3 -3 20 35.20 3.29 4 -6 -20 2.06 1.64 4 -6 -20 -0.73 2.31 -4 6 20 6.53 4.93 3 -5 -20 28.60 3.47 3 -5 -20 32.06 3.18 -3 5 20 32.09 6.57 2 -4 -20 36.71 4.00 2 -4 -20 43.62 3.80 1 -3 -20 46.80 4.63 -1 3 20 41.20 3.82 -1 3 20 53.09 8.57 0 -2 -20 76.50 6.31 0 2 20 69.52 5.82 0 2 20 65.36 10.08 -1 -1 -20 -4.13 1.90 1 1 20 -0.69 1.44 1 1 20 -2.12 7.75 -2 0 -20 87.22 7.10 2 0 20 59.91 12.03 2 0 20 86.86 6.90 -3 1 -20 9.60 2.14 3 -1 20 8.85 2.03 3 -1 20 15.80 6.85 -4 2 -20 0.00 1.90 4 -2 20 0.29 6.50 4 -2 20 -1.80 1.92 3 -7 -20 78.25 6.57 3 -7 -20 78.63 7.04 -3 7 20 77.33 8.75 2 -6 -20 18.02 2.21 2 -6 -20 14.91 2.90 -2 6 20 17.82 6.13 1 -5 -20 2.83 1.58 1 -5 -20 0.35 2.17 -1 5 20 1.90 6.36 -1 5 20 0.51 1.45 0 -4 -20 90.46 7.07 0 4 20 76.10 6.67 0 4 20 80.68 11.44 -1 -3 -20 -4.66 3.56 1 3 20 -0.12 1.61 2 2 20 13.53 13.97 2 2 20 18.70 2.41 -3 -1 -20 12.22 2.67 3 1 20 14.13 2.24 3 1 20 10.44 8.04 -4 0 -20 14.37 2.48 4 0 20 13.54 2.45 4 0 20 8.06 7.22 1 -7 -20 6.00 2.65 1 -7 -20 8.50 2.05 -1 7 20 5.62 6.08 -1 7 20 3.63 1.83 0 -6 -20 22.59 3.15 0 6 20 24.59 7.27 0 6 20 22.88 2.67 -1 -5 -20 5.62 2.27 1 5 20 3.96 7.25 1 5 20 5.28 1.92 -2 -4 -20 -4.24 2.05 2 4 20 -3.61 1.82 2 4 20 -5.86 7.46 -3 -3 -20 40.42 3.97 3 3 20 38.79 3.85 3 3 20 31.07 8.71 -4 -2 -20 0.89 2.35 4 2 20 -1.95 2.13 4 2 20 4.80 7.66 -1 -7 -20 42.70 4.97 1 7 20 49.92 4.75 1 7 20 41.42 8.33 -2 -6 -20 1.99 2.37 2 6 20 3.33 2.12 2 6 20 1.39 7.31 -3 -5 -20 16.52 2.85 3 5 20 5.05 7.81 5 3 -21 13.80 2.54 -5 -3 21 10.08 7.29 4 4 -21 -0.79 2.18 -4 -4 21 6.04 6.41 3 5 -21 36.92 3.59 -3 -5 21 24.02 6.72 2 6 -21 2.12 2.10 -2 -6 21 2.15 5.37 5 1 -21 -2.27 2.16 -5 -1 21 4.62 7.28 4 2 -21 -1.81 1.99 -4 -2 21 4.78 6.91 3 3 -21 9.45 2.31 -3 -3 21 11.20 6.67 2 4 -21 -3.09 1.92 -2 -4 21 2.41 5.65 1 5 -21 -1.06 1.87 -1 -5 21 2.28 5.41 0 -6 21 8.40 5.30 5 -1 -21 -1.06 2.11 -5 1 21 1.62 7.61 4 0 -21 -0.64 2.04 3 1 -21 0.65 3.65 -3 -1 21 8.30 9.49 2 2 -21 3.99 2.08 -2 -2 21 7.29 6.65 1 3 -21 5.64 1.99 -1 -3 21 14.02 6.11 0 4 -21 -2.51 1.76 0 -4 21 2.00 5.30 -1 5 -21 48.06 4.35 1 -5 21 46.34 4.08 1 -5 21 32.10 6.63 5 -3 -21 13.79 2.62 -5 3 21 12.89 5.96 4 -2 -21 -0.16 2.14 -4 2 21 4.16 7.32 3 -1 -21 6.62 2.22 -3 1 21 18.15 13.17 2 0 -21 -0.87 2.02 1 1 -21 76.05 6.53 -1 -1 21 85.87 11.26 0 2 -21 0.33 1.87 0 -2 21 -0.54 1.01 0 -2 21 11.54 6.07 -1 3 -21 25.76 2.80 1 -3 21 26.42 6.47 1 -3 21 24.48 2.39 -2 4 -21 37.24 3.82 2 -4 21 37.04 3.69 2 -4 21 30.70 6.65 4 -4 -21 -0.54 1.28 4 -4 -21 2.98 2.31 -4 4 21 4.84 6.13 3 -3 -21 8.74 2.46 3 -3 -21 10.47 1.36 -3 3 21 8.04 6.99 2 -2 -21 7.63 1.15 2 -2 -21 2.71 2.25 -2 2 21 16.73 8.57 1 -1 -21 73.65 6.29 -1 1 21 56.53 4.88 -1 1 21 73.70 10.77 0 0 -21 -2.11 1.95 0 0 21 0.21 7.22 0 0 21 -1.04 1.13 -1 1 -21 -1.12 1.79 1 -1 21 3.72 7.05 1 -1 21 -0.16 1.36 -2 2 -21 33.85 3.79 2 -2 21 37.69 7.45 2 -2 21 34.06 3.60 -3 3 -21 3.25 1.90 3 -3 21 3.96 1.88 3 -3 21 7.95 6.22 3 -5 -21 39.33 3.68 -3 5 21 33.43 7.30 2 -4 -21 -1.63 2.25 -2 4 21 -6.89 6.71 1 -3 -21 12.42 2.21 1 -3 -21 9.05 2.30 -1 3 21 3.80 1.62 -1 3 21 -1.33 7.76 0 -2 -21 2.89 2.18 0 2 21 1.94 2.06 0 2 21 2.38 7.98 -1 -1 -21 -0.84 3.37 1 1 21 -1.89 1.46 1 1 21 0.80 8.05 -2 0 -21 -4.80 3.68 2 0 21 -2.04 1.62 2 0 21 -2.77 7.15 -3 1 -21 25.77 2.98 3 -1 21 24.37 2.77 3 -1 21 19.85 7.50 2 -6 -21 5.02 1.69 2 -6 -21 0.79 2.59 -2 6 21 3.04 6.44 1 -5 -21 2.98 1.61 1 -5 -21 -0.55 2.28 -1 5 21 0.45 1.54 -1 5 21 0.40 7.24 0 -4 -21 -2.67 2.11 0 4 21 -9.59 7.63 0 4 21 -1.38 1.51 -1 -3 -21 25.85 3.24 1 3 21 17.71 8.51 1 3 21 31.57 2.93 -2 -2 -21 38.83 3.80 2 2 21 37.33 4.05 2 2 21 28.74 8.73 -3 -1 -21 27.25 3.14 3 1 21 16.50 8.20 3 1 21 25.32 2.93 0 -6 -21 37.06 3.79 0 6 21 31.25 3.29 0 6 21 22.07 7.99 -1 -5 -21 61.73 5.56 1 5 21 54.96 5.26 1 5 21 50.63 9.59 -2 -4 -21 43.04 4.53 2 4 21 41.23 4.47 2 4 21 36.10 9.09 -3 -3 -21 8.09 2.33 3 3 21 2.73 2.15 3 3 21 6.60 7.84 4 2 -22 26.65 3.28 -4 -2 22 24.63 7.83 3 3 -22 12.88 2.51 -3 -3 22 14.30 6.90 2 4 -22 22.92 3.09 -2 -4 22 19.39 6.59 1 5 -22 4.49 2.05 -1 -5 22 3.53 5.95 4 0 -22 34.95 3.74 -4 0 22 33.13 8.76 3 1 -22 3.93 2.21 -3 -1 22 3.51 7.73 2 2 -22 2.08 2.17 -2 -2 22 7.88 7.14 1 3 -22 -3.37 1.93 -1 -3 22 -1.68 6.04 0 4 -22 3.53 1.95 0 -4 22 7.42 5.83 4 -2 -22 28.89 3.48 -4 2 22 29.52 7.87 3 -1 -22 6.25 2.29 -3 1 22 12.30 8.33 2 0 -22 -1.06 2.13 -2 0 22 7.72 7.98 1 1 -22 -5.21 2.37 -1 -1 22 3.27 7.29 0 2 -22 6.79 2.21 0 -2 22 10.23 6.82 -1 3 -22 -2.53 1.85 1 -3 22 0.67 5.85 1 -3 22 -2.00 1.29 3 -3 -22 19.60 2.86 -3 3 22 14.09 7.83 2 -2 -22 1.89 1.23 2 -2 -22 -1.00 2.14 -2 2 22 1.31 7.96 1 -1 -22 -3.36 2.11 1 -1 -22 3.05 1.00 -1 1 22 -0.84 0.95 -1 1 22 -0.49 8.00 0 0 -22 60.52 5.07 0 0 22 46.51 4.35 0 0 22 62.11 9.51 -1 1 -22 -3.59 1.98 1 -1 22 -2.01 2.26 1 -1 22 9.32 7.12 -2 2 -22 -3.48 1.94 2 -2 22 -0.28 1.53 2 -2 22 10.41 6.87 2 -4 -22 25.13 3.46 2 -4 -22 31.25 2.99 -2 4 22 26.47 8.33 1 -3 -22 -0.13 1.38 1 -3 -22 -2.91 2.23 -1 3 22 -1.45 1.41 -1 3 22 -5.48 8.17 0 -2 -22 2.96 2.20 0 2 22 7.01 8.22 0 2 22 6.52 1.51 -1 -1 -22 0.14 2.03 1 1 22 1.09 8.10 1 1 22 0.84 1.54 -2 0 -22 0.14 2.04 2 0 22 0.63 1.70 2 0 22 -0.92 7.47 1 -5 -22 5.62 2.53 1 -5 -22 7.83 1.76 -1 5 22 2.39 1.64 -1 5 22 4.30 7.83 0 -4 -22 4.33 2.42 0 4 22 9.35 8.13 0 4 22 3.91 1.75 -1 -3 -22 -2.97 2.22 1 3 22 0.81 8.33 1 3 22 -1.93 1.71 -2 -2 -22 2.12 2.30 2 2 22 -0.38 1.81 2 2 22 -6.11 7.73 2 0 -23 -0.90 2.22 -2 0 23 3.93 7.93 1 1 -23 9.81 2.30 -1 -1 23 19.83 7.59 1 -1 -23 7.48 2.39 -1 1 23 15.20 8.24 0 0 -23 -3.95 1.99 0 0 23 5.14 7.60 0 0 0 0.00 0.00 ; _shelx_hkl_checksum 67454 _shelx_res_file ; TITL shelxt_a.res in C2/c shelx.res created by SHELXL-2018/3 at 12:17:42 on 10-Feb-2021 CELL 0.71073 8.3872 12.1039 18.1504 90.000 95.646 90.000 ZERR 4.00 0.0006 0.0006 0.0012 0.000 0.003 0.000 LATT 7 SYMM - X, Y, 1/2 - Z SFAC C H AL BR O UNIT 36 88 8 16 8 TEMP -173.13 L.S. 10 acta conf bond $h htab HTAB C2 Br1 EQIV $2 -x+1/2, -y+3/2, -z+1 HTAB C5 Br1_$2 WGHT 0.033700 0.046500 FVAR 0.08154 AL 3 0.116188 0.714229 0.329185 11.00000 0.01223 0.00618 = 0.01263 0.00071 0.00134 -0.00017 BR1 4 -0.028764 0.772399 0.423464 11.00000 0.02233 0.01703 = 0.01919 -0.00335 0.00634 0.00542 BR2 4 0.270350 0.857134 0.291581 11.00000 0.02347 0.01272 = 0.02788 0.00757 -0.00023 -0.00778 O1 5 0.272048 0.623885 0.380738 11.00000 0.01100 0.01017 = 0.01269 0.00284 0.00251 0.00115 C1 1 0.000000 0.632692 0.250000 10.50000 0.01630 0.00880 = 0.01410 0.00000 0.00113 0.00000 H1 2 -0.066075 0.588813 0.272269 11.00000 -1.20000 C2 1 0.243642 0.554995 0.444838 11.00000 0.01671 0.01506 = 0.01279 0.00445 -0.00012 0.00086 AFIX 23 H2A 2 0.204255 0.601947 0.483872 11.00000 -1.20000 H2B 2 0.345754 0.520776 0.465274 11.00000 -1.20000 AFIX 0 C3 1 0.122368 0.465506 0.423408 11.00000 0.01988 0.01594 = 0.02533 0.00419 0.00507 -0.00232 AFIX 137 H3A 2 0.111673 0.417489 0.466116 11.00000 -1.50000 H3B 2 0.158243 0.421669 0.382748 11.00000 -1.50000 H3C 2 0.018501 0.499297 0.407455 11.00000 -1.50000 AFIX 0 C4 1 0.405479 0.584246 0.340736 11.00000 0.01627 0.01426 = 0.01567 -0.00300 0.00636 0.00157 AFIX 23 H4A 2 0.388925 0.608372 0.288425 11.00000 -1.20000 H4B 2 0.408161 0.502482 0.341600 11.00000 -1.20000 AFIX 0 C5 1 0.561819 0.628790 0.375791 11.00000 0.01469 0.02569 = 0.02063 -0.00209 0.00587 0.00147 AFIX 137 H5A 2 0.650079 0.596834 0.351275 11.00000 -1.50000 H5B 2 0.574490 0.609271 0.428443 11.00000 -1.50000 H5C 2 0.563012 0.709361 0.370553 11.00000 -1.50000 AFIX 0 HKLF 4 REM shelxt_a.res in C2/c REM wR2 = 0.0759, GooF = S = 1.073, Restrained GooF = 1.073 for all data REM R1 = 0.0305 for 1736 Fo > 4sig(Fo) and 0.0396 for all 2027 data REM 83 parameters refined using 0 restraints END WGHT 0.0336 0.0837 REM Instructions for potential hydrogen bonds HTAB C2 Br1 HTAB C5 Br1_$2 REM Highest difference peak 0.744, deepest hole -0.726, 1-sigma level 0.135 Q1 1 0.3017 0.8531 0.3363 11.00000 0.05 0.74 Q2 1 0.0484 0.7479 0.4596 11.00000 0.05 0.70 Q3 1 0.1893 0.8794 0.2606 11.00000 0.05 0.66 Q4 1 -0.1124 0.7498 0.3856 11.00000 0.05 0.64 Q5 1 -0.0588 0.7732 0.3700 11.00000 0.05 0.60 Q6 1 0.2378 0.8419 0.2362 11.00000 0.05 0.59 Q7 1 0.0115 0.7807 0.4712 11.00000 0.05 0.59 Q8 1 -0.1120 0.7993 0.3878 11.00000 0.05 0.57 Q9 1 0.2106 0.6563 0.3649 11.00000 0.05 0.47 Q10 1 0.0565 0.6628 0.2788 11.00000 0.05 0.42 Q11 1 0.1569 0.4213 0.4578 11.00000 0.05 0.41 Q12 1 0.1115 0.8439 0.2198 11.00000 0.05 0.41 Q13 1 -0.1358 0.6920 0.4372 11.00000 0.05 0.37 Q14 1 0.2052 0.6024 0.3605 11.00000 0.05 0.36 Q15 1 0.7647 0.7177 0.3689 11.00000 0.05 0.35 Q16 1 0.3432 0.6344 0.4042 11.00000 0.05 0.35 Q17 1 0.5872 0.6403 0.4161 11.00000 0.05 0.35 Q18 1 0.4266 0.9431 0.2919 11.00000 0.05 0.34 Q19 1 0.3552 0.4947 0.5260 11.00000 0.05 0.34 Q20 1 0.3620 0.4244 0.3082 11.00000 0.05 0.33 ; _shelx_res_checksum 63807 loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, y, -z+1/2' 'x+1/2, y+1/2, z' '-x+1/2, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y, z-1/2' '-x+1/2, -y+1/2, -z' 'x+1/2, -y+1/2, z-1/2' loop_ _atom_site_type_symbol _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group Al Al 0.11619(11) 0.71423(7) 0.32918(6) 0.0103(2) Uani d 1 . . Br Br1 -0.02876(4) 0.77240(3) 0.42346(2) 0.01923(12) Uani d 1 . . Br Br2 0.27035(4) 0.85713(3) 0.29158(2) 0.02154(12) Uani d 1 . . O O1 0.2720(3) 0.62389(16) 0.38074(13) 0.0112(4) Uani d 1 . . C C1 0.000000 0.6327(3) 0.250000 0.0131(9) Uani d 1 . . H H1 -0.066(4) 0.589(3) 0.272(2) 0.016 Uiso d 1 . . C C2 0.2436(4) 0.5550(2) 0.44484(19) 0.0150(7) Uani d 1 . . H H2A 0.204255 0.601947 0.483872 0.018 Uiso calc 1 . . H H2B 0.345754 0.520776 0.465274 0.018 Uiso calc 1 . . C C3 0.1224(4) 0.4655(3) 0.4234(2) 0.0202(8) Uani d 1 . . H H3A 0.111673 0.417489 0.466116 0.030 Uiso calc 1 . . H H3B 0.158243 0.421669 0.382748 0.030 Uiso calc 1 . . H H3C 0.018501 0.499297 0.407455 0.030 Uiso calc 1 . . C C4 0.4055(4) 0.5842(3) 0.34074(19) 0.0151(7) Uani d 1 . . H H4A 0.388925 0.608372 0.288425 0.018 Uiso calc 1 . . H H4B 0.408161 0.502482 0.341600 0.018 Uiso calc 1 . . C C5 0.5618(4) 0.6288(3) 0.3758(2) 0.0201(7) Uani d 1 . . H H5A 0.650079 0.596834 0.351275 0.030 Uiso calc 1 . . H H5B 0.574490 0.609271 0.428443 0.030 Uiso calc 1 . . H H5C 0.563012 0.709361 0.370553 0.030 Uiso calc 1 . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Al 0.0122(5) 0.0062(4) 0.0126(5) -0.0002(3) 0.0013(4) 0.0007(3) Br1 0.0223(2) 0.01703(18) 0.0192(2) 0.00542(12) 0.00634(15) -0.00335(13) Br2 0.0235(2) 0.01272(17) 0.0279(2) -0.00778(12) -0.00023(15) 0.00757(13) O1 0.0110(11) 0.0102(10) 0.0127(12) 0.0012(8) 0.0025(9) 0.0028(8) C1 0.016(2) 0.0088(19) 0.014(2) 0.000 0.0011(19) 0.000 C2 0.0167(17) 0.0151(15) 0.0128(17) 0.0009(12) -0.0001(13) 0.0045(13) C3 0.0199(18) 0.0159(16) 0.025(2) -0.0023(13) 0.0051(15) 0.0042(14) C4 0.0163(17) 0.0143(14) 0.0157(17) 0.0016(12) 0.0064(14) -0.0030(13) C5 0.0147(18) 0.0257(17) 0.0206(19) 0.0015(13) 0.0059(14) -0.0021(14) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0033 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Al Al 0.0645 0.0514 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Br Br -0.2901 2.4595 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0106 0.0060 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag O1 Al C1 . . 110.42(13) y O1 Al Br2 . . 101.60(7) y C1 Al Br2 . . 114.90(9) y O1 Al Br1 . . 101.52(8) y C1 Al Br1 . . 116.44(5) y Br2 Al Br1 . . 110.07(4) y C2 O1 C4 . . 113.3(2) ? C2 O1 Al . . 124.38(19) ? C4 O1 Al . . 117.9(2) ? Al C1 Al . 2 118.4(2) ? Al C1 H1 . . 105(2) ? Al C1 H1 2 . 111(2) ? Al C1 H1 . 2 111(2) ? Al C1 H1 2 2 105(2) ? H1 C1 H1 . 2 107(5) ? O1 C2 C3 . . 111.1(3) ? O1 C2 H2A . . 109.4 ? C3 C2 H2A . . 109.4 ? O1 C2 H2B . . 109.4 ? C3 C2 H2B . . 109.4 ? H2A C2 H2B . . 108.0 ? C2 C3 H3A . . 109.5 ? C2 C3 H3B . . 109.5 ? H3A C3 H3B . . 109.5 ? C2 C3 H3C . . 109.5 ? H3A C3 H3C . . 109.5 ? H3B C3 H3C . . 109.5 ? O1 C4 C5 . . 110.4(3) ? O1 C4 H4A . . 109.6 ? C5 C4 H4A . . 109.6 ? O1 C4 H4B . . 109.6 ? C5 C4 H4B . . 109.6 ? H4A C4 H4B . . 108.1 ? C4 C5 H5A . . 109.5 ? C4 C5 H5B . . 109.5 ? H5A C5 H5B . . 109.5 ? C4 C5 H5C . . 109.5 ? H5A C5 H5C . . 109.5 ? H5B C5 H5C . . 109.5 ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag Al O1 . 1.881(2) y Al C1 . 1.927(2) y Al Br2 . 2.3029(9) y Al Br1 . 2.3046(10) y O1 C2 . 1.470(4) ? O1 C4 . 1.473(4) ? C1 H1 . 0.89(4) ? C1 H1 2 0.89(4) ? C2 C3 . 1.510(4) ? C2 H2A . 0.9900 ? C2 H2B . 0.9900 ? C3 H3A . 0.9800 ? C3 H3B . 0.9800 ? C3 H3C . 0.9800 ? C4 C5 . 1.500(5) ? C4 H4A . 0.9900 ? C4 H4B . 0.9900 ? C5 H5A . 0.9800 ? C5 H5B . 0.9800 ? C5 H5C . 0.9800 ? loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_site_symmetry_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA _geom_hbond_publ_flag C2 H2A Br1 . 0.99 2.98 3.481(3) 112.8 yes C5 H5B Br1 7_566 0.98 3.10 3.871(4) 136.3 yes loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion _geom_torsion_publ_flag C1 Al O1 C2 . . . . -89.5(2) ? Br2 Al O1 C2 . . . . 148.1(2) ? Br1 Al O1 C2 . . . . 34.6(2) ? C1 Al O1 C4 . . . . 65.4(2) ? Br2 Al O1 C4 . . . . -57.0(2) ? Br1 Al O1 C4 . . . . -170.52(18) ? C4 O1 C2 C3 . . . . -91.5(3) ? Al O1 C2 C3 . . . . 64.4(3) ? C2 O1 C4 C5 . . . . -85.6(3) ? Al O1 C4 C5 . . . . 116.9(3) ? _cod_database_fobs_code 2243837