#------------------------------------------------------------------------------ #$Date: 2020-06-05 14:26:55 +0300 (Fri, 05 Jun 2020) $ #$Revision: 252901 $ #$URL: file:///home/coder/svn-repositories/cod/cif/7/15/74/7157464.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/ # # All data on this site have been placed in the public domain by the # contributors. # data_7157464 loop_ _publ_author_name 'Dos Santos, Emerson E. F.' 'de Souza, Gabriela F. P.' 'Simoni, Deborah A.' 'Salles, Jr, Airton G' _publ_section_title ; A base-promoted tandem approach to bicyclic 8-membered ring ketones. ; _journal_issue 17 _journal_name_full 'Organic & biomolecular chemistry' _journal_page_first 3249 _journal_page_last 3253 _journal_paper_doi 10.1039/d0ob00618a _journal_volume 18 _journal_year 2020 _chemical_formula_moiety 'C22 H18 O2' _chemical_formula_sum 'C22 H18 O2' _chemical_formula_weight 314.36 _chemical_name_systematic (4Z)-2,4-diphenyl-8,9-dihydrocycloocta[b]furan-6(7H)-one _space_group_crystal_system monoclinic _space_group_IT_number 14 _space_group_name_Hall '-P 2ybc' _space_group_name_H-M_alt 'P 1 21/c 1' _atom_sites_solution_hydrogens geom _audit_block_doi 10.5517/ccdc.csd.cc21hcpm _audit_creation_method SHELXL-2014 _audit_update_record ; 2019-01-17 deposited with the CCDC. 2020-04-08 downloaded from the CCDC. ; _cell_angle_alpha 90 _cell_angle_beta 97.281(4) _cell_angle_gamma 90 _cell_formula_units_Z 4 _cell_length_a 8.6541(5) _cell_length_b 5.7809(3) _cell_length_c 33.543(2) _cell_measurement_reflns_used 92 _cell_measurement_temperature 150(2) _cell_measurement_theta_max 36.79 _cell_measurement_theta_min 9.28 _cell_volume 1664.57(16) _computing_cell_refinement 'SAINT (Bruker, 2010)' _computing_data_collection 'APEX2 (Bruker, 2010)' _computing_data_reduction 'SAINT (Bruker, 2010)' _computing_structure_refinement 'SHELXL-2014/7 (Sheldrick, 2015)' _computing_structure_solution 'SHELXS-97 (Sheldrick, 2008)' _diffrn_ambient_temperature 150(2) _diffrn_detector_area_resol_mean 8.3333 _diffrn_measured_fraction_theta_full 0.854 _diffrn_measured_fraction_theta_max 0.837 _diffrn_measurement_device_type 'Bruker APEX CCD detector' _diffrn_measurement_method 'phi and omega scans' _diffrn_radiation_source 'fine-focus sealed tube' _diffrn_radiation_type CuK\a _diffrn_radiation_wavelength 1.54178 _diffrn_reflns_av_R_equivalents 0.0604 _diffrn_reflns_av_unetI/netI 0.0657 _diffrn_reflns_Laue_measured_fraction_full 0.854 _diffrn_reflns_Laue_measured_fraction_max 0.837 _diffrn_reflns_limit_h_max 9 _diffrn_reflns_limit_h_min -10 _diffrn_reflns_limit_k_max 6 _diffrn_reflns_limit_k_min -5 _diffrn_reflns_limit_l_max 39 _diffrn_reflns_limit_l_min -39 _diffrn_reflns_number 6055 _diffrn_reflns_point_group_measured_fraction_full 0.854 _diffrn_reflns_point_group_measured_fraction_max 0.837 _diffrn_reflns_theta_full 67.679 _diffrn_reflns_theta_max 68.820 _diffrn_reflns_theta_min 5.152 _exptl_absorpt_coefficient_mu 0.624 _exptl_absorpt_correction_T_max 0.7531 _exptl_absorpt_correction_T_min 0.6111 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details 'SADABS (Bruker, 2010)' _exptl_crystal_colour COLORLESS _exptl_crystal_density_diffrn 1.254 _exptl_crystal_description PLATE _exptl_crystal_F_000 664 _exptl_crystal_recrystallization_method 'Re-crystallisation from solvent: acetone and water' _exptl_crystal_size_max 0.238 _exptl_crystal_size_mid 0.178 _exptl_crystal_size_min 0.032 _refine_diff_density_max 0.151 _refine_diff_density_min -0.177 _refine_diff_density_rms 0.038 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.130 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 217 _refine_ls_number_reflns 2583 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.130 _refine_ls_R_factor_all 0.0751 _refine_ls_R_factor_gt 0.0584 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+1.1175P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1262 _refine_ls_wR_factor_ref 0.1326 _reflns_Friedel_coverage 0.000 _reflns_number_gt 2018 _reflns_number_total 2583 _reflns_threshold_expression 'I > 2\s(I)' _cod_data_source_file d0ob00618a2.cif _cod_data_source_block FUR-A _cod_depositor_comments 'Adding full bibliography for 7157464.cif.' _cod_original_cell_volume 1664.55(16) _cod_original_sg_symbol_H-M 'P 21/c' _cod_database_code 7157464 _publcif_datablock.id {d9bb4aa3-109e-40ba-bc30-91ae974a3651} _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _shelx_estimated_absorpt_t_min 0.866 _shelx_estimated_absorpt_t_max 0.980 _shelxl_version_number 2014-3 _shelx_res_file ; TITL FUR-A.res in P2(1)/c REM Old TITL FUR-A in P2(1)/c REM SHELXT solution in P2(1)/c REM R1 0.131, Rweak 0.027, Alpha 0.039, Orientation as input REM Formula found by SHELXT: C22 O2 CELL 1.54178 8.6541 5.7809 33.5426 90.000 97.281 90.000 ZERR 4.000 0.0005 0.0003 0.0020 0.000 0.004 0.000 LATT 1 SYMM -X, 1/2+Y, 1/2-Z SFAC C H O UNIT 88 72 8 TEMP -123.150 SIZE 0.032 0.178 0.238 L.S. 20 ACTA BOND $H OMIT 6 0 0 LIST 6 CONF FMAP 2 PLAN 5 WGHT 0.000000 1.117500 FVAR 0.64111 O1 3 0.695648 0.640419 0.358114 11.00000 0.03168 0.02722 = 0.04003 0.00090 0.00564 -0.00372 O2 3 0.641721 0.267786 0.514804 11.00000 0.05055 0.04300 = 0.03838 0.00468 0.00100 -0.00454 C1 1 0.778234 0.682719 0.278350 11.00000 0.03755 0.03633 = 0.04084 0.00383 0.00095 -0.00383 AFIX 43 H1 2 0.805456 0.805229 0.296785 11.00000 -1.20000 AFIX 0 C2 1 0.829413 0.687770 0.240989 11.00000 0.03979 0.03964 = 0.04664 0.00808 0.00569 -0.00545 AFIX 43 H2 2 0.890596 0.813896 0.233799 11.00000 -1.20000 AFIX 0 C3 1 0.791400 0.508180 0.213865 11.00000 0.03872 0.04833 = 0.03826 0.00608 0.00715 -0.00080 AFIX 43 H3 2 0.828030 0.509755 0.188339 11.00000 -1.20000 AFIX 0 C4 1 0.700120 0.327855 0.224330 11.00000 0.04317 0.04719 = 0.04115 -0.00215 0.00557 -0.00290 AFIX 43 H4 2 0.672229 0.206945 0.205614 11.00000 -1.20000 AFIX 0 C5 1 0.648818 0.320848 0.261622 11.00000 0.03774 0.03309 = 0.04406 0.00006 0.00574 -0.00578 AFIX 43 H5 2 0.587396 0.194403 0.268567 11.00000 -1.20000 AFIX 0 C6 1 0.687298 0.500528 0.289358 11.00000 0.02495 0.03324 = 0.03919 0.00484 0.00177 0.00122 C7 1 0.632906 0.484379 0.328807 11.00000 0.02791 0.03063 = 0.03640 0.00115 -0.00033 -0.00044 C8 1 0.533638 0.342906 0.344509 11.00000 0.02748 0.03095 = 0.03748 0.00231 0.00224 -0.00216 AFIX 43 H8 2 0.473855 0.223202 0.330619 11.00000 -1.20000 AFIX 0 C9 1 0.533572 0.404115 0.386003 11.00000 0.02666 0.02516 = 0.03872 0.00258 0.00291 0.00054 C10 1 0.633846 0.586474 0.392431 11.00000 0.03105 0.02675 = 0.03938 0.00184 0.00598 0.00227 C11 1 0.687359 0.718692 0.429784 11.00000 0.04356 0.02978 = 0.04379 -0.00439 0.01160 -0.00867 AFIX 23 H11A 2 0.598257 0.742700 0.445147 11.00000 -1.20000 H11B 2 0.725321 0.872586 0.422465 11.00000 -1.20000 AFIX 0 C12 1 0.818557 0.591409 0.456463 11.00000 0.04077 0.04536 = 0.04130 -0.00157 0.00423 -0.01315 AFIX 23 H12A 2 0.917298 0.610551 0.444803 11.00000 -1.20000 H12B 2 0.832262 0.662898 0.483500 11.00000 -1.20000 AFIX 0 C13 1 0.785376 0.334027 0.460570 11.00000 0.03377 0.04029 = 0.04224 0.00075 -0.00057 -0.00093 AFIX 23 H13A 2 0.778251 0.260885 0.433712 11.00000 -1.20000 H13B 2 0.873571 0.261620 0.477804 11.00000 -1.20000 AFIX 0 C14 1 0.636271 0.286869 0.478438 11.00000 0.04110 0.02181 = 0.03830 0.00171 0.00295 -0.00135 C15 1 0.484233 0.258741 0.453738 11.00000 0.03450 0.02635 = 0.04085 0.00010 0.00818 -0.00220 AFIX 43 H15 2 0.403933 0.201744 0.467944 11.00000 -1.20000 AFIX 0 C16 1 0.439368 0.300103 0.414332 11.00000 0.03311 0.02052 = 0.03882 -0.00268 0.00596 0.00046 C17 1 0.274244 0.247489 0.397418 11.00000 0.02905 0.02872 = 0.03574 -0.00178 0.00747 0.00214 C18 1 0.190867 0.409760 0.372531 11.00000 0.03304 0.02928 = 0.04487 0.00248 0.00818 0.00188 AFIX 43 H18 2 0.239689 0.549316 0.365909 11.00000 -1.20000 AFIX 0 C19 1 0.036800 0.367628 0.357444 11.00000 0.03295 0.03991 = 0.04762 -0.00002 0.00434 0.00846 AFIX 43 H19 2 -0.020051 0.479939 0.340896 11.00000 -1.20000 AFIX 0 C20 1 -0.034695 0.163593 0.366289 11.00000 0.02681 0.04450 = 0.04681 -0.00428 0.00680 0.00084 AFIX 43 H20 2 -0.140341 0.135668 0.355908 11.00000 -1.20000 AFIX 0 C21 1 0.048495 0.000005 0.390369 11.00000 0.03617 0.03704 = 0.04613 0.00051 0.01127 -0.00655 AFIX 43 H21 2 0.000490 -0.141969 0.396045 11.00000 -1.20000 AFIX 0 C22 1 0.202209 0.043021 0.406274 11.00000 0.03320 0.03380 = 0.03986 0.00424 0.00685 -0.00178 AFIX 43 H22 2 0.258024 -0.068246 0.423277 11.00000 -1.20000 AFIX 0 HKLF 4 REM FUR-A.res in P2(1)/c REM R1 = 0.0584 for 2018 Fo > 4sig(Fo) and 0.0751 for all 2583 data REM 217 parameters refined using 0 restraints END WGHT 0.0000 1.1175 REM Highest difference peak 0.151, deepest hole -0.177, 1-sigma level 0.038 Q1 1 0.0984 0.2584 0.3455 11.00000 0.05 0.15 Q2 1 0.4365 0.5398 0.4024 11.00000 0.05 0.15 Q3 1 0.5243 0.1596 0.4305 11.00000 0.05 0.14 Q4 1 0.5014 0.3825 0.5231 11.00000 0.05 0.14 Q5 1 0.2491 0.2101 0.4256 11.00000 0.05 0.13 ; _shelx_res_checksum 67838 loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y-1/2, z-1/2' loop_ _atom_site_label _atom_site_type_symbol _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_occupancy _atom_site_site_symmetry_order _atom_site_calc_flag _atom_site_refinement_flags_posn _atom_site_refinement_flags_adp _atom_site_refinement_flags_occupancy _atom_site_disorder_assembly _atom_site_disorder_group O1 O 0.69565(19) 0.6404(3) 0.35811(5) 0.0329(4) Uani 1 1 d . . . . . O2 O 0.6417(2) 0.2678(4) 0.51480(5) 0.0444(5) Uani 1 1 d . . . . . C1 C 0.7782(3) 0.6827(5) 0.27835(8) 0.0386(6) Uani 1 1 d . . . . . H1 H 0.8055 0.8052 0.2968 0.046 Uiso 1 1 calc R U . . . C2 C 0.8294(3) 0.6878(5) 0.24099(8) 0.0420(7) Uani 1 1 d . . . . . H2 H 0.8906 0.8139 0.2338 0.050 Uiso 1 1 calc R U . . . C3 C 0.7914(3) 0.5082(5) 0.21387(8) 0.0416(7) Uani 1 1 d . . . . . H3 H 0.8280 0.5098 0.1883 0.050 Uiso 1 1 calc R U . . . C4 C 0.7001(3) 0.3279(6) 0.22433(8) 0.0438(7) Uani 1 1 d . . . . . H4 H 0.6722 0.2069 0.2056 0.053 Uiso 1 1 calc R U . . . C5 C 0.6488(3) 0.3208(5) 0.26162(8) 0.0383(6) Uani 1 1 d . . . . . H5 H 0.5874 0.1944 0.2686 0.046 Uiso 1 1 calc R U . . . C6 C 0.6873(3) 0.5005(5) 0.28936(7) 0.0327(6) Uani 1 1 d . . . . . C7 C 0.6329(3) 0.4844(5) 0.32881(7) 0.0320(6) Uani 1 1 d . . . . . C8 C 0.5336(3) 0.3429(5) 0.34451(7) 0.0321(6) Uani 1 1 d . . . . . H8 H 0.4739 0.2232 0.3306 0.039 Uiso 1 1 calc R U . . . C9 C 0.5336(3) 0.4041(4) 0.38600(7) 0.0303(5) Uani 1 1 d . . . . . C10 C 0.6338(3) 0.5865(5) 0.39243(7) 0.0323(6) Uani 1 1 d . . . . . C11 C 0.6874(3) 0.7187(5) 0.42978(7) 0.0385(6) Uani 1 1 d . . . . . H11A H 0.5983 0.7427 0.4451 0.046 Uiso 1 1 calc R U . . . H11B H 0.7253 0.8726 0.4225 0.046 Uiso 1 1 calc R U . . . C12 C 0.8186(3) 0.5914(5) 0.45646(8) 0.0426(7) Uani 1 1 d . . . . . H12A H 0.9173 0.6106 0.4448 0.051 Uiso 1 1 calc R U . . . H12B H 0.8323 0.6629 0.4835 0.051 Uiso 1 1 calc R U . . . C13 C 0.7854(3) 0.3340(5) 0.46057(8) 0.0392(6) Uani 1 1 d . . . . . H13A H 0.7783 0.2609 0.4337 0.047 Uiso 1 1 calc R U . . . H13B H 0.8736 0.2616 0.4778 0.047 Uiso 1 1 calc R U . . . C14 C 0.6363(3) 0.2869(4) 0.47844(7) 0.0339(6) Uani 1 1 d . . . . . C15 C 0.4842(3) 0.2587(4) 0.45374(7) 0.0336(6) Uani 1 1 d . . . . . H15 H 0.4039 0.2017 0.4679 0.040 Uiso 1 1 calc R U . . . C16 C 0.4394(3) 0.3001(4) 0.41433(7) 0.0307(5) Uani 1 1 d . . . . . C17 C 0.2742(3) 0.2475(5) 0.39742(7) 0.0309(5) Uani 1 1 d . . . . . C18 C 0.1909(3) 0.4098(5) 0.37253(7) 0.0354(6) Uani 1 1 d . . . . . H18 H 0.2397 0.5493 0.3659 0.043 Uiso 1 1 calc R U . . . C19 C 0.0368(3) 0.3676(5) 0.35744(8) 0.0402(6) Uani 1 1 d . . . . . H19 H -0.0201 0.4799 0.3409 0.048 Uiso 1 1 calc R U . . . C20 C -0.0347(3) 0.1636(5) 0.36629(8) 0.0392(6) Uani 1 1 d . . . . . H20 H -0.1403 0.1357 0.3559 0.047 Uiso 1 1 calc R U . . . C21 C 0.0485(3) 0.0000(5) 0.39037(8) 0.0393(6) Uani 1 1 d . . . . . H21 H 0.0005 -0.1420 0.3960 0.047 Uiso 1 1 calc R U . . . C22 C 0.2022(3) 0.0430(5) 0.40627(7) 0.0354(6) Uani 1 1 d . . . . . H22 H 0.2580 -0.0682 0.4233 0.043 Uiso 1 1 calc R U . . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_23 _atom_site_aniso_U_13 _atom_site_aniso_U_12 O1 0.0317(9) 0.0272(10) 0.0400(9) 0.0009(7) 0.0056(7) -0.0037(7) O2 0.0506(12) 0.0430(12) 0.0384(10) 0.0047(8) 0.0010(8) -0.0045(9) C1 0.0375(14) 0.0363(16) 0.0408(13) 0.0038(11) 0.0009(11) -0.0038(12) C2 0.0398(15) 0.0396(17) 0.0466(14) 0.0081(12) 0.0057(11) -0.0054(13) C3 0.0387(15) 0.0483(18) 0.0383(13) 0.0061(12) 0.0072(11) -0.0008(13) C4 0.0432(16) 0.0472(18) 0.0411(14) -0.0021(13) 0.0056(12) -0.0029(13) C5 0.0377(14) 0.0331(15) 0.0441(14) 0.0001(11) 0.0057(11) -0.0058(12) C6 0.0249(12) 0.0332(15) 0.0392(13) 0.0048(11) 0.0018(10) 0.0012(10) C7 0.0279(12) 0.0306(14) 0.0364(12) 0.0012(10) -0.0003(10) -0.0004(11) C8 0.0275(12) 0.0309(14) 0.0375(12) 0.0023(10) 0.0022(10) -0.0022(10) C9 0.0267(12) 0.0252(13) 0.0387(12) 0.0026(10) 0.0029(9) 0.0005(10) C10 0.0311(13) 0.0268(14) 0.0394(13) 0.0018(10) 0.0060(10) 0.0023(10) C11 0.0436(15) 0.0298(15) 0.0438(14) -0.0044(11) 0.0116(11) -0.0087(12) C12 0.0408(15) 0.0454(18) 0.0413(14) -0.0016(12) 0.0042(11) -0.0132(13) C13 0.0338(14) 0.0403(17) 0.0422(13) 0.0007(12) -0.0006(10) -0.0009(12) C14 0.0411(14) 0.0218(14) 0.0383(13) 0.0017(10) 0.0029(10) -0.0014(11) C15 0.0345(14) 0.0264(14) 0.0409(13) 0.0001(11) 0.0082(10) -0.0022(10) C16 0.0331(13) 0.0205(13) 0.0388(13) -0.0027(10) 0.0060(10) 0.0005(10) C17 0.0291(12) 0.0287(14) 0.0357(12) -0.0018(10) 0.0075(9) 0.0021(10) C18 0.0330(14) 0.0293(14) 0.0449(13) 0.0025(11) 0.0082(10) 0.0019(11) C19 0.0330(14) 0.0399(17) 0.0476(14) 0.0000(12) 0.0043(11) 0.0085(12) C20 0.0268(13) 0.0445(17) 0.0468(14) -0.0043(12) 0.0068(10) 0.0008(12) C21 0.0362(14) 0.0370(16) 0.0461(14) 0.0005(12) 0.0113(11) -0.0065(12) C22 0.0332(14) 0.0338(15) 0.0399(13) 0.0042(11) 0.0068(10) -0.0018(11) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0181 0.0091 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0492 0.0322 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle_publ_flag C10 O1 C7 106.73(19) . . ? C2 C1 C6 120.9(3) . . ? C2 C1 H1 119.5 . . ? C6 C1 H1 119.5 . . ? C1 C2 C3 120.0(3) . . ? C1 C2 H2 120.0 . . ? C3 C2 H2 120.0 . . ? C4 C3 C2 119.5(3) . . ? C4 C3 H3 120.2 . . ? C2 C3 H3 120.2 . . ? C5 C4 C3 120.9(3) . . ? C5 C4 H4 119.6 . . ? C3 C4 H4 119.6 . . ? C4 C5 C6 120.1(3) . . ? C4 C5 H5 119.9 . . ? C6 C5 H5 119.9 . . ? C1 C6 C5 118.5(2) . . ? C1 C6 C7 123.1(2) . . ? C5 C6 C7 118.4(2) . . ? C8 C7 O1 109.2(2) . . ? C8 C7 C6 133.6(2) . . ? O1 C7 C6 117.1(2) . . ? C7 C8 C9 108.0(2) . . ? C7 C8 H8 126.0 . . ? C9 C8 H8 126.0 . . ? C10 C9 C8 105.4(2) . . ? C10 C9 C16 127.8(2) . . ? C8 C9 C16 126.8(2) . . ? C9 C10 O1 110.6(2) . . ? C9 C10 C11 130.7(2) . . ? O1 C10 C11 118.6(2) . . ? C10 C11 C12 111.8(2) . . ? C10 C11 H11A 109.3 . . ? C12 C11 H11A 109.3 . . ? C10 C11 H11B 109.3 . . ? C12 C11 H11B 109.3 . . ? H11A C11 H11B 107.9 . . ? C13 C12 C11 112.7(2) . . ? C13 C12 H12A 109.1 . . ? C11 C12 H12A 109.1 . . ? C13 C12 H12B 109.1 . . ? C11 C12 H12B 109.1 . . ? H12A C12 H12B 107.8 . . ? C14 C13 C12 113.0(2) . . ? C14 C13 H13A 109.0 . . ? C12 C13 H13A 109.0 . . ? C14 C13 H13B 109.0 . . ? C12 C13 H13B 109.0 . . ? H13A C13 H13B 107.8 . . ? O2 C14 C15 118.1(2) . . ? O2 C14 C13 119.0(2) . . ? C15 C14 C13 122.9(2) . . ? C16 C15 C14 131.0(2) . . ? C16 C15 H15 114.5 . . ? C14 C15 H15 114.5 . . ? C15 C16 C9 126.6(2) . . ? C15 C16 C17 118.4(2) . . ? C9 C16 C17 114.9(2) . . ? C22 C17 C18 119.3(2) . . ? C22 C17 C16 121.6(2) . . ? C18 C17 C16 119.1(2) . . ? C19 C18 C17 120.1(3) . . ? C19 C18 H18 120.0 . . ? C17 C18 H18 120.0 . . ? C20 C19 C18 120.5(3) . . ? C20 C19 H19 119.7 . . ? C18 C19 H19 119.7 . . ? C19 C20 C21 119.6(2) . . ? C19 C20 H20 120.2 . . ? C21 C20 H20 120.2 . . ? C20 C21 C22 120.2(3) . . ? C20 C21 H21 119.9 . . ? C22 C21 H21 119.9 . . ? C17 C22 C21 120.3(2) . . ? C17 C22 H22 119.9 . . ? C21 C22 H22 119.9 . . ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_distance _geom_bond_site_symmetry_2 _geom_bond_publ_flag O1 C10 1.365(3) . ? O1 C7 1.393(3) . ? O2 C14 1.220(3) . ? C1 C2 1.381(4) . ? C1 C6 1.392(4) . ? C1 H1 0.9500 . ? C2 C3 1.392(4) . ? C2 H2 0.9500 . ? C3 C4 1.380(4) . ? C3 H3 0.9500 . ? C4 C5 1.380(4) . ? C4 H4 0.9500 . ? C5 C6 1.406(4) . ? C5 H5 0.9500 . ? C6 C7 1.463(4) . ? C7 C8 1.341(4) . ? C8 C9 1.436(4) . ? C8 H8 0.9500 . ? C9 C10 1.365(4) . ? C9 C16 1.458(4) . ? C10 C11 1.490(4) . ? C11 C12 1.541(4) . ? C11 H11A 0.9900 . ? C11 H11B 0.9900 . ? C12 C13 1.525(4) . ? C12 H12A 0.9900 . ? C12 H12B 0.9900 . ? C13 C14 1.515(4) . ? C13 H13A 0.9900 . ? C13 H13B 0.9900 . ? C14 C15 1.472(3) . ? C15 C16 1.351(3) . ? C15 H15 0.9500 . ? C16 C17 1.500(3) . ? C17 C22 1.386(4) . ? C17 C18 1.395(3) . ? C18 C19 1.386(4) . ? C18 H18 0.9500 . ? C19 C20 1.382(4) . ? C19 H19 0.9500 . ? C20 C21 1.385(4) . ? C20 H20 0.9500 . ? C21 C22 1.391(4) . ? C21 H21 0.9500 . ? C22 H22 0.9500 . ? loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion_publ_flag C6 C1 C2 C3 -0.6(4) . . . . ? C1 C2 C3 C4 1.2(4) . . . . ? C2 C3 C4 C5 -1.4(4) . . . . ? C3 C4 C5 C6 1.0(4) . . . . ? C2 C1 C6 C5 0.2(4) . . . . ? C2 C1 C6 C7 178.7(2) . . . . ? C4 C5 C6 C1 -0.4(4) . . . . ? C4 C5 C6 C7 -178.9(2) . . . . ? C10 O1 C7 C8 1.2(3) . . . . ? C10 O1 C7 C6 -177.3(2) . . . . ? C1 C6 C7 C8 171.9(3) . . . . ? C5 C6 C7 C8 -9.6(4) . . . . ? C1 C6 C7 O1 -10.0(4) . . . . ? C5 C6 C7 O1 168.5(2) . . . . ? O1 C7 C8 C9 -1.4(3) . . . . ? C6 C7 C8 C9 176.8(3) . . . . ? C7 C8 C9 C10 1.1(3) . . . . ? C7 C8 C9 C16 178.1(2) . . . . ? C8 C9 C10 O1 -0.3(3) . . . . ? C16 C9 C10 O1 -177.3(2) . . . . ? C8 C9 C10 C11 -177.2(3) . . . . ? C16 C9 C10 C11 5.8(4) . . . . ? C7 O1 C10 C9 -0.5(3) . . . . ? C7 O1 C10 C11 176.8(2) . . . . ? C9 C10 C11 C12 80.8(3) . . . . ? O1 C10 C11 C12 -95.8(3) . . . . ? C10 C11 C12 C13 -44.7(3) . . . . ? C11 C12 C13 C14 -59.1(3) . . . . ? C12 C13 C14 O2 -90.4(3) . . . . ? C12 C13 C14 C15 90.7(3) . . . . ? O2 C14 C15 C16 169.9(3) . . . . ? C13 C14 C15 C16 -11.2(4) . . . . ? C14 C15 C16 C9 -5.1(5) . . . . ? C14 C15 C16 C17 178.4(3) . . . . ? C10 C9 C16 C15 -40.8(4) . . . . ? C8 C9 C16 C15 142.8(3) . . . . ? C10 C9 C16 C17 135.8(3) . . . . ? C8 C9 C16 C17 -40.6(4) . . . . ? C15 C16 C17 C22 -45.0(3) . . . . ? C9 C16 C17 C22 138.0(2) . . . . ? C15 C16 C17 C18 134.2(3) . . . . ? C9 C16 C17 C18 -42.7(3) . . . . ? C22 C17 C18 C19 1.1(4) . . . . ? C16 C17 C18 C19 -178.2(2) . . . . ? C17 C18 C19 C20 -1.1(4) . . . . ? C18 C19 C20 C21 -0.1(4) . . . . ? C19 C20 C21 C22 1.4(4) . . . . ? C18 C17 C22 C21 0.2(4) . . . . ? C16 C17 C22 C21 179.5(2) . . . . ? C20 C21 C22 C17 -1.4(4) . . . . ? loop_ _publcif_info_exptl_table_extra_item sin_theta_over_lambda_max loop_ _publcif_info_exptl_table_header_item ?